Type-II Weyl nodes, flat bands, and evidence for a topological Hall-effect in the new ferromagnet FeCr$_3$Te$_6$

Fuente: arXiv
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Main Authors: Karullithodi, Shyam Raj, Kulichenko, Vadym, Plata, Mario A., Ptok, Andrzej, Lee, Sang-Eon, McCandless, Gregory T., Chan, Julia Y., Balicas, Luis
Format: Preprint
Published: 2025
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author Karullithodi, Shyam Raj
Kulichenko, Vadym
Plata, Mario A.
Ptok, Andrzej
Lee, Sang-Eon
McCandless, Gregory T.
Chan, Julia Y.
Balicas, Luis
author_facet Karullithodi, Shyam Raj
Kulichenko, Vadym
Plata, Mario A.
Ptok, Andrzej
Lee, Sang-Eon
McCandless, Gregory T.
Chan, Julia Y.
Balicas, Luis
contents The interplay between linearly dispersing or Dirac-like, and flat electronic bands, for instance, in the kagome ferromagnets, has attracted attention due to a possible interplay between topology and electronic correlations. Here, we report the synthesis, structural, electrical, and magnetic properties of a single-crystalline ferromagnetic compound, namely Fe$_{1/3}$CrTe$_2$ or FeCr$_3$Te$_6$, which crystallizes in the $P\bar{3}m1$ space group instead of the $I2/m$ previously reported for FeCr$_2$Te$_4$. Electronic band structure calculations reveal type-II Dirac nodes and relatively flat bands near the Fermi level ($\varepsilon_F$). This compound shows onset Curie temperature $T_{\text{c}}\simeq 120$ K, followed by an additional ferromagnetic transition near $T_{\text{c2}} \sim 92.5 $ K. Below $T_{\text{c}}$, FeCr$_3$Te$_6$ displays a pronounced anomalous Hall effect, as well as sizable coercive fields that exceed $μ_0H = 1$~T at low $T$s. However, a scaling analysis indicates that the anomalous Hall effect results from a significant intrinsic contribution, as expected from the calculations, but also from the extrinsic mechanism, i.e., scattering. The extrinsic contribution probably results from occupational disorder at the 1b Fe-site within the van der Waals gap of the CrTe$_2$ host. We also observe evidence for a topological Hall component superimposed onto the overall Hall response, suggesting the presence of chiral spin textures akin to skyrmions in this centrosymmetric system. Their possible presence will require experimental confirmation.
format Preprint
id arxiv_https___arxiv_org_abs_2504_17035
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Type-II Weyl nodes, flat bands, and evidence for a topological Hall-effect in the new ferromagnet FeCr$_3$Te$_6$
Karullithodi, Shyam Raj
Kulichenko, Vadym
Plata, Mario A.
Ptok, Andrzej
Lee, Sang-Eon
McCandless, Gregory T.
Chan, Julia Y.
Balicas, Luis
Other Condensed Matter
The interplay between linearly dispersing or Dirac-like, and flat electronic bands, for instance, in the kagome ferromagnets, has attracted attention due to a possible interplay between topology and electronic correlations. Here, we report the synthesis, structural, electrical, and magnetic properties of a single-crystalline ferromagnetic compound, namely Fe$_{1/3}$CrTe$_2$ or FeCr$_3$Te$_6$, which crystallizes in the $P\bar{3}m1$ space group instead of the $I2/m$ previously reported for FeCr$_2$Te$_4$. Electronic band structure calculations reveal type-II Dirac nodes and relatively flat bands near the Fermi level ($\varepsilon_F$). This compound shows onset Curie temperature $T_{\text{c}}\simeq 120$ K, followed by an additional ferromagnetic transition near $T_{\text{c2}} \sim 92.5 $ K. Below $T_{\text{c}}$, FeCr$_3$Te$_6$ displays a pronounced anomalous Hall effect, as well as sizable coercive fields that exceed $μ_0H = 1$~T at low $T$s. However, a scaling analysis indicates that the anomalous Hall effect results from a significant intrinsic contribution, as expected from the calculations, but also from the extrinsic mechanism, i.e., scattering. The extrinsic contribution probably results from occupational disorder at the 1b Fe-site within the van der Waals gap of the CrTe$_2$ host. We also observe evidence for a topological Hall component superimposed onto the overall Hall response, suggesting the presence of chiral spin textures akin to skyrmions in this centrosymmetric system. Their possible presence will require experimental confirmation.
title Type-II Weyl nodes, flat bands, and evidence for a topological Hall-effect in the new ferromagnet FeCr$_3$Te$_6$
topic Other Condensed Matter
url https://arxiv.org/abs/2504.17035