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Main Authors: Song, Xinru, Bu, Xiaoyu, Zhao, Xiaohui, Zhang, Rongxiang, Wang, Shang, Dong, Fulong
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2504.17335
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author Song, Xinru
Bu, Xiaoyu
Zhao, Xiaohui
Zhang, Rongxiang
Wang, Shang
Dong, Fulong
author_facet Song, Xinru
Bu, Xiaoyu
Zhao, Xiaohui
Zhang, Rongxiang
Wang, Shang
Dong, Fulong
contents We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the tight-binding approximation. The orientation-dependent harmonic spectra exhibit pronounced enhancement of specific harmonics, which we attribute to the caustic effect. Using the recombination trajectory model, we reveal that the orientation dependence of these enhanced harmonics originates from the distinct band structures encountered by electrons ionized from the two inequivalent $\textrm{K}$ points. Moreover, we focus on the ellipticity of the enhanced harmonics at specific angles and demonstrate that it primarily depends on the phase difference between the parallel and perpendicular components, which can be accurately predicted by our recombination trajectory model. Based on these insights, we propose a two-color (fundamental plus second-harmonic) field scheme to generate isolated elliptically polarized attosecond pulses (IEAPs) in gapped graphene. Our findings may provide a promising pathway toward the generation of IEAPs in gapped graphene or transition metal dichalcogenides.
format Preprint
id arxiv_https___arxiv_org_abs_2504_17335
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Isolated elliptically-polarized attosecond pulse generation in gapped graphene driven by linearly polarized laser fields
Song, Xinru
Bu, Xiaoyu
Zhao, Xiaohui
Zhang, Rongxiang
Wang, Shang
Dong, Fulong
Atomic Physics
We theoretically investigate high-order harmonic generation (HHG) and its ellipticity in gapped graphene, driven by a femtosecond short-pulse laser at various orientation angles, employing the two-band density-matrix equations within the tight-binding approximation. The orientation-dependent harmonic spectra exhibit pronounced enhancement of specific harmonics, which we attribute to the caustic effect. Using the recombination trajectory model, we reveal that the orientation dependence of these enhanced harmonics originates from the distinct band structures encountered by electrons ionized from the two inequivalent $\textrm{K}$ points. Moreover, we focus on the ellipticity of the enhanced harmonics at specific angles and demonstrate that it primarily depends on the phase difference between the parallel and perpendicular components, which can be accurately predicted by our recombination trajectory model. Based on these insights, we propose a two-color (fundamental plus second-harmonic) field scheme to generate isolated elliptically polarized attosecond pulses (IEAPs) in gapped graphene. Our findings may provide a promising pathway toward the generation of IEAPs in gapped graphene or transition metal dichalcogenides.
title Isolated elliptically-polarized attosecond pulse generation in gapped graphene driven by linearly polarized laser fields
topic Atomic Physics
url https://arxiv.org/abs/2504.17335