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Main Authors: Ding, Qing-Ping, Taylor, Charles, Lee, Yongbin, Dissanayake, Charuni, Mishra, Vireshwar, Le, Dang Khoa, Phan, Manh-Huong, Nakajima, Yasuyuki, Furukawa, Yuji
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2504.18924
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author Ding, Qing-Ping
Taylor, Charles
Lee, Yongbin
Dissanayake, Charuni
Mishra, Vireshwar
Le, Dang Khoa
Phan, Manh-Huong
Nakajima, Yasuyuki
Furukawa, Yuji
author_facet Ding, Qing-Ping
Taylor, Charles
Lee, Yongbin
Dissanayake, Charuni
Mishra, Vireshwar
Le, Dang Khoa
Phan, Manh-Huong
Nakajima, Yasuyuki
Furukawa, Yuji
contents Static and dynamical magnetic and electronic properties of the kagome metal Sc$_3$Mn$_3$Al$_7$Si$_5$ have been investigated by $^{27}$Al nuclear magnetic resonance (NMR) measurements. The temperature dependence of Knight shift ($K$) shows a similar temperature dependence of the DC magnetic susceptibility $χ$ except for the low-temperature region below $\sim$ 50 K where $K$ is almost constant while $χ$ keeps increasing, which suggests that the increase in $χ$ at low temperatures is not intrinsic. $^{27}$Al spin-lattice relaxation rate divided by temperature ($1/T_1T$) is found to be constant, confirming the metallic state of Sc$_3$Mn$_3$Al$_7$Si$_5$ from a microscopic point of view. Based on a Korringa ratio analysis using the $T_1$ and $K$ data, ferromagnetic spin fluctuations are found to dominate in Sc$_3$Mn$_3$Al$_7$Si$_5$. These fluctuations are suggested to be very slow with frequencies on the order of kilohertz or lower.
format Preprint
id arxiv_https___arxiv_org_abs_2504_18924
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Slow ferromagnetic fluctuations in the kagome metal Sc$_3$Mn$_3$Al$_7$Si$_5$ revealed by $^{27}$Al NMR
Ding, Qing-Ping
Taylor, Charles
Lee, Yongbin
Dissanayake, Charuni
Mishra, Vireshwar
Le, Dang Khoa
Phan, Manh-Huong
Nakajima, Yasuyuki
Furukawa, Yuji
Strongly Correlated Electrons
Static and dynamical magnetic and electronic properties of the kagome metal Sc$_3$Mn$_3$Al$_7$Si$_5$ have been investigated by $^{27}$Al nuclear magnetic resonance (NMR) measurements. The temperature dependence of Knight shift ($K$) shows a similar temperature dependence of the DC magnetic susceptibility $χ$ except for the low-temperature region below $\sim$ 50 K where $K$ is almost constant while $χ$ keeps increasing, which suggests that the increase in $χ$ at low temperatures is not intrinsic. $^{27}$Al spin-lattice relaxation rate divided by temperature ($1/T_1T$) is found to be constant, confirming the metallic state of Sc$_3$Mn$_3$Al$_7$Si$_5$ from a microscopic point of view. Based on a Korringa ratio analysis using the $T_1$ and $K$ data, ferromagnetic spin fluctuations are found to dominate in Sc$_3$Mn$_3$Al$_7$Si$_5$. These fluctuations are suggested to be very slow with frequencies on the order of kilohertz or lower.
title Slow ferromagnetic fluctuations in the kagome metal Sc$_3$Mn$_3$Al$_7$Si$_5$ revealed by $^{27}$Al NMR
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2504.18924