Bio-Derived Graphite from Pterocarpus marsupium Leaves for rGO-MoO$_3$ Nanocomposites with Enhanced Photocatalytic Efficiency

Fuente: arXiv
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Main Authors: Mary, P. Princeya, Kumaresavanji, M., Venkatesh, P. Sundara, Kannan, N., Vasumathi, V.
Format: Preprint
Published: 2025
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author Mary, P. Princeya
Kumaresavanji, M.
Venkatesh, P. Sundara
Kannan, N.
Vasumathi, V.
author_facet Mary, P. Princeya
Kumaresavanji, M.
Venkatesh, P. Sundara
Kannan, N.
Vasumathi, V.
contents This study presents a sustainable approach to synthesize bio-graphite from Pterocarpus marsupium (Indian Kino) leaves without using chemical catalysts, activating agents, or organic solvents. The resulting bio-graphite was used to produce reduced graphene oxide (rGO) via a modified Hummers method. The bio-graphite derived rGO was further incorporated with orthorhombic structured MoO$_3$ at different percentages (1, 3, and 6 wt.%) using ultrasonication. Structural, morphological, and functional characterizations were conducted using XRD, FESEM, FTIR, and UV-Vis DRS spectroscopy, revealing a bandgap of 2.82 eV for the rGO(3 wt.%)-MoO$_3$ composite. Photocatalytic activity was evaluated via methylene blue degradation under natural sunlight. The rGO(3 wt.%)-MoO$_3$ nanocomposite showed superior performance, achieving 90% degradation in 150 minutes when compared to 65% by pure MoO$_3$. The Scavenger tests confirmed superoxide radicals $(\cdot O_2^-)$ as the main reactive species. This work highlights the potential of bio-graphite derived rGO-MoO$_3$ nanocomposites as efficient, eco-friendly photocatalysts for wastewater treatment.
format Preprint
id arxiv_https___arxiv_org_abs_2504_19758
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Bio-Derived Graphite from Pterocarpus marsupium Leaves for rGO-MoO$_3$ Nanocomposites with Enhanced Photocatalytic Efficiency
Mary, P. Princeya
Kumaresavanji, M.
Venkatesh, P. Sundara
Kannan, N.
Vasumathi, V.
Materials Science
This study presents a sustainable approach to synthesize bio-graphite from Pterocarpus marsupium (Indian Kino) leaves without using chemical catalysts, activating agents, or organic solvents. The resulting bio-graphite was used to produce reduced graphene oxide (rGO) via a modified Hummers method. The bio-graphite derived rGO was further incorporated with orthorhombic structured MoO$_3$ at different percentages (1, 3, and 6 wt.%) using ultrasonication. Structural, morphological, and functional characterizations were conducted using XRD, FESEM, FTIR, and UV-Vis DRS spectroscopy, revealing a bandgap of 2.82 eV for the rGO(3 wt.%)-MoO$_3$ composite. Photocatalytic activity was evaluated via methylene blue degradation under natural sunlight. The rGO(3 wt.%)-MoO$_3$ nanocomposite showed superior performance, achieving 90% degradation in 150 minutes when compared to 65% by pure MoO$_3$. The Scavenger tests confirmed superoxide radicals $(\cdot O_2^-)$ as the main reactive species. This work highlights the potential of bio-graphite derived rGO-MoO$_3$ nanocomposites as efficient, eco-friendly photocatalysts for wastewater treatment.
title Bio-Derived Graphite from Pterocarpus marsupium Leaves for rGO-MoO$_3$ Nanocomposites with Enhanced Photocatalytic Efficiency
topic Materials Science
url https://arxiv.org/abs/2504.19758