Fiber laser based stimulated Raman photothermal microscopy with long working distance optics

Fuente: arXiv
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Main Authors: Ge, Xiaowei, Zhu, Yifan, Sun, Dingcheng, Ni, Hongli, Li, Yueming, Dessai, Chinmayee V. Prabhu, Cheng, Ji-Xin
Format: Preprint
Published: 2025
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author Ge, Xiaowei
Zhu, Yifan
Sun, Dingcheng
Ni, Hongli
Li, Yueming
Dessai, Chinmayee V. Prabhu
Cheng, Ji-Xin
author_facet Ge, Xiaowei
Zhu, Yifan
Sun, Dingcheng
Ni, Hongli
Li, Yueming
Dessai, Chinmayee V. Prabhu
Cheng, Ji-Xin
contents Stimulated Raman scattering (SRS) microscopy is a highly sensitive chemical imaging technique. However, the broader application of SRS has been limited by two key challenges: the reliance on low-noise but bulky solid-state laser sources and stringent sample requirements necessitated by high numerical aperture (NA) optics. Here, we present a fiber laser based stimulated Raman photothermal (SRP) microscope that addresses these limitations. While appreciating the portability and compactness of a noisy source, fiber laser SRP enables a two-order-of-magnitude improvement in signal to noise ratio over fiber laser SRS without balance detection. Furthermore, with the use of low NA, long working distance optics for signal collection, SRP expands the allowed sample space from millimeters to centimeters, which diversifies the sample formats to multi-well plates and thick tissues. The sensitivity and imaging depth are further amplified by using urea for both thermal enhancement and tissue clearance. Together, fiber laser SRP microscopy provides a robust, user-friendly platform for diverse applications.
format Preprint
id arxiv_https___arxiv_org_abs_2504_19875
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Fiber laser based stimulated Raman photothermal microscopy with long working distance optics
Ge, Xiaowei
Zhu, Yifan
Sun, Dingcheng
Ni, Hongli
Li, Yueming
Dessai, Chinmayee V. Prabhu
Cheng, Ji-Xin
Optics
Instrumentation and Detectors
Stimulated Raman scattering (SRS) microscopy is a highly sensitive chemical imaging technique. However, the broader application of SRS has been limited by two key challenges: the reliance on low-noise but bulky solid-state laser sources and stringent sample requirements necessitated by high numerical aperture (NA) optics. Here, we present a fiber laser based stimulated Raman photothermal (SRP) microscope that addresses these limitations. While appreciating the portability and compactness of a noisy source, fiber laser SRP enables a two-order-of-magnitude improvement in signal to noise ratio over fiber laser SRS without balance detection. Furthermore, with the use of low NA, long working distance optics for signal collection, SRP expands the allowed sample space from millimeters to centimeters, which diversifies the sample formats to multi-well plates and thick tissues. The sensitivity and imaging depth are further amplified by using urea for both thermal enhancement and tissue clearance. Together, fiber laser SRP microscopy provides a robust, user-friendly platform for diverse applications.
title Fiber laser based stimulated Raman photothermal microscopy with long working distance optics
topic Optics
Instrumentation and Detectors
url https://arxiv.org/abs/2504.19875