Twist Engineering of Anisotropic Excitonic and Optical Properties of a Two-Dimensional Magnetic Semiconductor

Fuente: arXiv
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Autori principali: Li, Qiuyang, Wan, Xiaohan, Li, Senlei, Alfrey, Adam, Liu, Wenhao, Zhai, Zixin, Alpers, Wyatt, Yang, Yujie, Wladyszewska, Irmina, Beach, Christiano W., Zhao, Liuyan, Lv, Bing, Du, Chunhui Rita, Sun, Kai, Deng, Hui
Natura: Preprint
Pubblicazione: 2025
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author Li, Qiuyang
Wan, Xiaohan
Li, Senlei
Alfrey, Adam
Liu, Wenhao
Zhai, Zixin
Alpers, Wyatt
Yang, Yujie
Wladyszewska, Irmina
Beach, Christiano W.
Zhao, Liuyan
Lv, Bing
Du, Chunhui Rita
Sun, Kai
Deng, Hui
author_facet Li, Qiuyang
Wan, Xiaohan
Li, Senlei
Alfrey, Adam
Liu, Wenhao
Zhai, Zixin
Alpers, Wyatt
Yang, Yujie
Wladyszewska, Irmina
Beach, Christiano W.
Zhao, Liuyan
Lv, Bing
Du, Chunhui Rita
Sun, Kai
Deng, Hui
contents Two dimensional (2D) van der Waals (vdW) magnetic semiconductors are a new class of quantum materials for studying the emergent physics of excitons and spins in the 2D limit. Twist engineering provides a powerful tool to manipulate the fundamental properties of 2D vdW materials. Here, we show that twist engineering of the anisotropic ferromagnetic monolayer semiconductor, CrSBr, leads to bilayer magnetic semiconductors with continuously tunable magnetic moment, dielectric anisotropy, exciton energy and linear dichroism. We furthermore provide a model for exciton energy in the media with tunable anisotropy. These results advance fundamental studies on 2D vdW materials and open doors to applications to nano-optics, twistronics, and spintronics.
format Preprint
id arxiv_https___arxiv_org_abs_2505_00123
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Twist Engineering of Anisotropic Excitonic and Optical Properties of a Two-Dimensional Magnetic Semiconductor
Li, Qiuyang
Wan, Xiaohan
Li, Senlei
Alfrey, Adam
Liu, Wenhao
Zhai, Zixin
Alpers, Wyatt
Yang, Yujie
Wladyszewska, Irmina
Beach, Christiano W.
Zhao, Liuyan
Lv, Bing
Du, Chunhui Rita
Sun, Kai
Deng, Hui
Mesoscale and Nanoscale Physics
Materials Science
Two dimensional (2D) van der Waals (vdW) magnetic semiconductors are a new class of quantum materials for studying the emergent physics of excitons and spins in the 2D limit. Twist engineering provides a powerful tool to manipulate the fundamental properties of 2D vdW materials. Here, we show that twist engineering of the anisotropic ferromagnetic monolayer semiconductor, CrSBr, leads to bilayer magnetic semiconductors with continuously tunable magnetic moment, dielectric anisotropy, exciton energy and linear dichroism. We furthermore provide a model for exciton energy in the media with tunable anisotropy. These results advance fundamental studies on 2D vdW materials and open doors to applications to nano-optics, twistronics, and spintronics.
title Twist Engineering of Anisotropic Excitonic and Optical Properties of a Two-Dimensional Magnetic Semiconductor
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2505.00123