Stable self-charged perovskite quantum rods for liquid laser with near-zero threshold
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arXiv
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| Auteurs principaux: | , , , , , , , , , , , , , , , , , , , , |
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| Format: | Preprint |
| Publié: |
2025
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| _version_ | 1866912357032132608 |
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| author | Li, Jialu Han, Xue Wang, Wenjie Wang, Jinhui Zhang, Tingting Wu, Yuting Zhang, Guofeng Li, Bin Yang, Changgang Guo, Wenli Zhang, Mi Chen, Ruiyun Qin, Chengbing Hu, Jianyong Yang, Zhichun Liu, Shaoding Wang, Yue Gao, Yunan Ma, Jie Xiao, Liantuan Jia, Suotang |
| author_facet | Li, Jialu Han, Xue Wang, Wenjie Wang, Jinhui Zhang, Tingting Wu, Yuting Zhang, Guofeng Li, Bin Yang, Changgang Guo, Wenli Zhang, Mi Chen, Ruiyun Qin, Chengbing Hu, Jianyong Yang, Zhichun Liu, Shaoding Wang, Yue Gao, Yunan Ma, Jie Xiao, Liantuan Jia, Suotang |
| contents | Colloidal quantum dots (QDs) are promising optical gain materials that require further threshold reduction to realize their full potential. While QD charging theoretically reduces the threshold to zero, its effectiveness has been limited by strong Auger recombination and unstable charging. Here we theoretically reveal the optimal combination of charging number and Auger recombination to minimize the lasing threshold. Experimentally, we develop stable self-charged perovskite quantum rods (QRs) as an alternative to QDs via state engineering and Mn-doping strategy. An unprecedented two-order-of-magnitude reduction in nonradiative Auger recombination enables QRs to support a sufficient charging number of up to 6. The QR liquid lasing is then achieved with a near-zero threshold of 0.098 using quasi-continuous pumping of nanosecond pulses, which is the lowest threshold among all reported QD lasers. These achievements demonstrate the potential of the specially engineered QRs as an excellent gain media and pave the way for their prospective applications. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2505_00464 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Stable self-charged perovskite quantum rods for liquid laser with near-zero threshold Li, Jialu Han, Xue Wang, Wenjie Wang, Jinhui Zhang, Tingting Wu, Yuting Zhang, Guofeng Li, Bin Yang, Changgang Guo, Wenli Zhang, Mi Chen, Ruiyun Qin, Chengbing Hu, Jianyong Yang, Zhichun Liu, Shaoding Wang, Yue Gao, Yunan Ma, Jie Xiao, Liantuan Jia, Suotang Mesoscale and Nanoscale Physics Applied Physics Optics Colloidal quantum dots (QDs) are promising optical gain materials that require further threshold reduction to realize their full potential. While QD charging theoretically reduces the threshold to zero, its effectiveness has been limited by strong Auger recombination and unstable charging. Here we theoretically reveal the optimal combination of charging number and Auger recombination to minimize the lasing threshold. Experimentally, we develop stable self-charged perovskite quantum rods (QRs) as an alternative to QDs via state engineering and Mn-doping strategy. An unprecedented two-order-of-magnitude reduction in nonradiative Auger recombination enables QRs to support a sufficient charging number of up to 6. The QR liquid lasing is then achieved with a near-zero threshold of 0.098 using quasi-continuous pumping of nanosecond pulses, which is the lowest threshold among all reported QD lasers. These achievements demonstrate the potential of the specially engineered QRs as an excellent gain media and pave the way for their prospective applications. |
| title | Stable self-charged perovskite quantum rods for liquid laser with near-zero threshold |
| topic | Mesoscale and Nanoscale Physics Applied Physics Optics |
| url | https://arxiv.org/abs/2505.00464 |