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Main Authors: Brassington, A., Ma, Q., Duan, G., Calder, S., Kolesnikov, A. I., Taddei, K. M., Sala, G., Choi, E. S., Wang, H., Xie, W., Frandsen, B. A., Li, N., Sun, X. F., Liu, C., Yu, R., Zhou, H. D., Aczel, A. A.
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2505.00766
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author Brassington, A.
Ma, Q.
Duan, G.
Calder, S.
Kolesnikov, A. I.
Taddei, K. M.
Sala, G.
Choi, E. S.
Wang, H.
Xie, W.
Frandsen, B. A.
Li, N.
Sun, X. F.
Liu, C.
Yu, R.
Zhou, H. D.
Aczel, A. A.
author_facet Brassington, A.
Ma, Q.
Duan, G.
Calder, S.
Kolesnikov, A. I.
Taddei, K. M.
Sala, G.
Choi, E. S.
Wang, H.
Xie, W.
Frandsen, B. A.
Li, N.
Sun, X. F.
Liu, C.
Yu, R.
Zhou, H. D.
Aczel, A. A.
contents The quantum dimer magnet, with antiferromagnetic intradimer and interdimer Heisenberg exchange between spin-1/2 moments, is known to host an up/down - down/up singlet ground state when the intradimer exchange is dominant. Rare-earth-based quantum dimer systems with strong spin-orbit coupling offer the opportunity for tuning their magnetic properties by using magnetic anisotropy as a control knob. Here, we present bulk characterization and neutron scattering measurements of the quantum dimer magnet Yb$_2$Be$_2$SiO$_7$. We find that the Yb$^{3+}$ ions can be described by an effective spin-1/2 model at low temperatures and the system does not show signs of magnetic order down to 50 mK. The magnetization, heat capacity, and neutron spectroscopy data can be well-described by an isolated dimer model with highly anisotropic exchange that stabilizes a singlet ground state with a wavefunction up/up - down/down or up/up + down/down. Our results show that strong spin-orbit coupling can induce novel entangled states of matter in quantum dimer magnets.
format Preprint
id arxiv_https___arxiv_org_abs_2505_00766
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Novel bipartite entanglement in the quantum dimer magnet Yb$_2$Be$_2$SiO$_7$
Brassington, A.
Ma, Q.
Duan, G.
Calder, S.
Kolesnikov, A. I.
Taddei, K. M.
Sala, G.
Choi, E. S.
Wang, H.
Xie, W.
Frandsen, B. A.
Li, N.
Sun, X. F.
Liu, C.
Yu, R.
Zhou, H. D.
Aczel, A. A.
Strongly Correlated Electrons
The quantum dimer magnet, with antiferromagnetic intradimer and interdimer Heisenberg exchange between spin-1/2 moments, is known to host an up/down - down/up singlet ground state when the intradimer exchange is dominant. Rare-earth-based quantum dimer systems with strong spin-orbit coupling offer the opportunity for tuning their magnetic properties by using magnetic anisotropy as a control knob. Here, we present bulk characterization and neutron scattering measurements of the quantum dimer magnet Yb$_2$Be$_2$SiO$_7$. We find that the Yb$^{3+}$ ions can be described by an effective spin-1/2 model at low temperatures and the system does not show signs of magnetic order down to 50 mK. The magnetization, heat capacity, and neutron spectroscopy data can be well-described by an isolated dimer model with highly anisotropic exchange that stabilizes a singlet ground state with a wavefunction up/up - down/down or up/up + down/down. Our results show that strong spin-orbit coupling can induce novel entangled states of matter in quantum dimer magnets.
title Novel bipartite entanglement in the quantum dimer magnet Yb$_2$Be$_2$SiO$_7$
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2505.00766