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Bibliographic Details
Main Authors: Imamura, Kumpei, Namba, Ryuichi, Ishioka, Riku, Ishihara, Kota, Matsuda, Yuji, Lee, Seunghun, Moon, Eun-Gook, Hashimoto, Kenichiro, Shibauchi, Takasada
Format: Preprint
Published: 2025
Subjects:
Online Access:https://arxiv.org/abs/2505.00971
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Table of Contents:
  • The spin-orbit coupled Mott insulator $α$-RuCl$_3$ has emerged as a prime candidate for realizing the Kitaev quantum spin liquid (KQSL), characterized by Majorana quasiparticles, whose edge states exhibit a distinctive half-integer quantized thermal Hall conductivity. However, its van der Waals nature makes its thermal Hall response highly sensitive to structural disorder, leading to sample-dependent variations. Here, we investigate low-energy bulk excitations in the field-induced quantum disordered (FIQD) state of newly available ultraclean single crystals of $α$-RuCl$_3$. High-resolution specific heat measurements under in-plane magnetic field rotation reveal an anisotropic excitation gap, whose field dependence is consistent with the Majorana gap in the KQSL state. Remarkably, when the field aligns with Ru-Ru bond directions, we observe gapless excitations with Dirac-like dispersions that quantitatively match theoretical predictions of Majorana bands based on the reported Kitaev interactions. Our findings in these ultraclean crystals provide strong evidence that the FIQD state of $α$-RuCl$_3$ is a robust KQSL, resilient against small disorder perturbations.