Unconventional orbital currents and torques due to ferro-rotational orbital textures

Fuente: arXiv
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Main Authors: Jo, Daegeun, Oppeneer, Peter M.
Format: Preprint
Published: 2025
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author Jo, Daegeun
Oppeneer, Peter M.
author_facet Jo, Daegeun
Oppeneer, Peter M.
contents Orbital angular momentum transport has emerged as a promising route for manipulating magnetic devices, yet its generation has largely relied on the conventional orbital Hall effect. Here, we show that ferro-rotational order enables the electrical generation of unconventional orbital currents. These orbital currents represent the orbital counterparts of spin currents due to ferromagnetic order, but arise from rotation-induced symmetry breaking rather than time-reversal symmetry breaking or spin-orbit coupling. Using tight-binding models, we identify the underlying intrinsic, nonrelativistic mechanism categorized as an electric hexadecapole moment and corroborate our findings with first-principles calculations for the ferro-rotational material TiAu$_4$. We further show that these rotation-induced orbital currents lead to surface orbital accumulation and unconventional orbital torque in a ferro-rotational/ferromagnetic metallic bilayer, allowing deterministic field-free switching. Our findings unveil a novel pathway for generating orbital currents beyond the conventional orbital Hall effect, broadening the landscape of orbitronics research to include novel ferroic materials and higher-order electric multipoles.
format Preprint
id arxiv_https___arxiv_org_abs_2505_04363
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Unconventional orbital currents and torques due to ferro-rotational orbital textures
Jo, Daegeun
Oppeneer, Peter M.
Materials Science
Mesoscale and Nanoscale Physics
Orbital angular momentum transport has emerged as a promising route for manipulating magnetic devices, yet its generation has largely relied on the conventional orbital Hall effect. Here, we show that ferro-rotational order enables the electrical generation of unconventional orbital currents. These orbital currents represent the orbital counterparts of spin currents due to ferromagnetic order, but arise from rotation-induced symmetry breaking rather than time-reversal symmetry breaking or spin-orbit coupling. Using tight-binding models, we identify the underlying intrinsic, nonrelativistic mechanism categorized as an electric hexadecapole moment and corroborate our findings with first-principles calculations for the ferro-rotational material TiAu$_4$. We further show that these rotation-induced orbital currents lead to surface orbital accumulation and unconventional orbital torque in a ferro-rotational/ferromagnetic metallic bilayer, allowing deterministic field-free switching. Our findings unveil a novel pathway for generating orbital currents beyond the conventional orbital Hall effect, broadening the landscape of orbitronics research to include novel ferroic materials and higher-order electric multipoles.
title Unconventional orbital currents and torques due to ferro-rotational orbital textures
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2505.04363