Mid-infrared quantum scanning microscopy via visible light beyond spatial correlations

Fuente: arXiv
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Autores principales: León-Torres, Josué R., Dosan, Vasile-Laurentiu, Ćurčić, Marija M., Lagarrigue, Alek, Setzpfandt, Frank, Gräfe, Markus, Gili, Valerio Flavio
Formato: Preprint
Publicado: 2025
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author León-Torres, Josué R.
Dosan, Vasile-Laurentiu
Ćurčić, Marija M.
Lagarrigue, Alek
Setzpfandt, Frank
Gräfe, Markus
Gili, Valerio Flavio
author_facet León-Torres, Josué R.
Dosan, Vasile-Laurentiu
Ćurčić, Marija M.
Lagarrigue, Alek
Setzpfandt, Frank
Gräfe, Markus
Gili, Valerio Flavio
contents The mid-infrared (MIR) region of the electromagnetic spectrum spans from 2- to 25-$μ\mathrm{m}$, serving as a valuable tool for accessing rich chemical information. Functional groups, lipids, and other complex molecules can be analyzed by optical absorption measurements due to their vibrational modes in the MIR spectral region. Over the past few decades, this field has faced challenges due to difficulties in generating MIR light and the limited maturity of detection systems in this spectral range. Quantum imaging with undetected light (QIUL) provides a spectrally tuneable photon-pair source, in which the sample can be illuminated with MIR light while visible (VIS) light is employed for detection and image reconstruction, overcoming the detection limitations and benefiting from the rich chemical information of the MIR spectral region. All previous QIUL implementations are based on spatial correlations, which are never perfect and thus hindered the imaging performance. In this work, we implement a raster-scanning QIUL method that is independent of the strength of the spatial correlations and achieves a spatial resolution beyond the limitations of these correlations.
format Preprint
id arxiv_https___arxiv_org_abs_2505_04490
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Mid-infrared quantum scanning microscopy via visible light beyond spatial correlations
León-Torres, Josué R.
Dosan, Vasile-Laurentiu
Ćurčić, Marija M.
Lagarrigue, Alek
Setzpfandt, Frank
Gräfe, Markus
Gili, Valerio Flavio
Optics
The mid-infrared (MIR) region of the electromagnetic spectrum spans from 2- to 25-$μ\mathrm{m}$, serving as a valuable tool for accessing rich chemical information. Functional groups, lipids, and other complex molecules can be analyzed by optical absorption measurements due to their vibrational modes in the MIR spectral region. Over the past few decades, this field has faced challenges due to difficulties in generating MIR light and the limited maturity of detection systems in this spectral range. Quantum imaging with undetected light (QIUL) provides a spectrally tuneable photon-pair source, in which the sample can be illuminated with MIR light while visible (VIS) light is employed for detection and image reconstruction, overcoming the detection limitations and benefiting from the rich chemical information of the MIR spectral region. All previous QIUL implementations are based on spatial correlations, which are never perfect and thus hindered the imaging performance. In this work, we implement a raster-scanning QIUL method that is independent of the strength of the spatial correlations and achieves a spatial resolution beyond the limitations of these correlations.
title Mid-infrared quantum scanning microscopy via visible light beyond spatial correlations
topic Optics
url https://arxiv.org/abs/2505.04490