Identifying optimal magnetic field configurations for decoherence mitigation of boron vacancies in hexagonal boron nitride

Fuente: arXiv
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Main Authors: Mistri, Basanta, Mahajan, Saksham, Donaldson, Felix, Kamineni, Rama K., Dhomkar, Siddharth
Format: Preprint
Published: 2025
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_version_ 1866914211432497152
author Mistri, Basanta
Mahajan, Saksham
Donaldson, Felix
Kamineni, Rama K.
Dhomkar, Siddharth
author_facet Mistri, Basanta
Mahajan, Saksham
Donaldson, Felix
Kamineni, Rama K.
Dhomkar, Siddharth
contents The negatively charged boron vacancy center in 2D hexagonal boron nitride has emerged as a promising quantum sensor. However, its sensitivity is constrained due to ubiquitous nuclear spins in the environment. The nuclear spins, hyperfine coupled with the central electron spin, effectively behave as magnetic field fluctuators, leading to rapid decoherence. Here, we explore the effectiveness of static magnetic field strength and orientation in realizing peculiar subspaces that can lead to enhanced spin coherence. Specifically, using detailed numerical simulations of the spin Hamiltonian, we identify specific field configurations that minimize energy gradients and, consequently, are expected to facilitate decoherence suppression. We also develop an approximate analytical model based on the perturbation theory that accurately predicts these low-gradient subspaces for magnetic fields aligned with the electron spin quantization axis, applicable not only to boron vacancies but to any spin-1 electronic system coupled to nearby nuclear spins. Furthermore, to stimulate experimental validation, we estimate coherence lifetimes as a function of various bias field configurations and demonstrate that significant decoherence suppression can indeed be achieved in certain regions. These findings and the developed methodology offer valuable insights for mitigating decoherence in a low-field regime.
format Preprint
id arxiv_https___arxiv_org_abs_2505_06574
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Identifying optimal magnetic field configurations for decoherence mitigation of boron vacancies in hexagonal boron nitride
Mistri, Basanta
Mahajan, Saksham
Donaldson, Felix
Kamineni, Rama K.
Dhomkar, Siddharth
Quantum Physics
Mesoscale and Nanoscale Physics
The negatively charged boron vacancy center in 2D hexagonal boron nitride has emerged as a promising quantum sensor. However, its sensitivity is constrained due to ubiquitous nuclear spins in the environment. The nuclear spins, hyperfine coupled with the central electron spin, effectively behave as magnetic field fluctuators, leading to rapid decoherence. Here, we explore the effectiveness of static magnetic field strength and orientation in realizing peculiar subspaces that can lead to enhanced spin coherence. Specifically, using detailed numerical simulations of the spin Hamiltonian, we identify specific field configurations that minimize energy gradients and, consequently, are expected to facilitate decoherence suppression. We also develop an approximate analytical model based on the perturbation theory that accurately predicts these low-gradient subspaces for magnetic fields aligned with the electron spin quantization axis, applicable not only to boron vacancies but to any spin-1 electronic system coupled to nearby nuclear spins. Furthermore, to stimulate experimental validation, we estimate coherence lifetimes as a function of various bias field configurations and demonstrate that significant decoherence suppression can indeed be achieved in certain regions. These findings and the developed methodology offer valuable insights for mitigating decoherence in a low-field regime.
title Identifying optimal magnetic field configurations for decoherence mitigation of boron vacancies in hexagonal boron nitride
topic Quantum Physics
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2505.06574