Resonant Self-Diffraction of Femtosecond Extreme Ultraviolet Pulses in Cobalt

Fuente: arXiv
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Main Authors: Maznev, Alexei A., Lee, Wonseok, Cushing, Scott K., De Angelis, Dario, Fainozzi, Danny, Foglia, Laura, Gutt, Christian, Jaouen, Nicolas, Kammerbauer, Fabian, Masciovecchio, Claudio, Mincigrucci, Riccardo, Nelson, Keith A., Paltanin, Ettore, Pelli-Cresi, Jacopo Stefano, Polewczyk, Vincent, Ksenzov, Dmitriy, Bencivenga, Filippo
Format: Preprint
Published: 2025
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author Maznev, Alexei A.
Lee, Wonseok
Cushing, Scott K.
De Angelis, Dario
Fainozzi, Danny
Foglia, Laura
Gutt, Christian
Jaouen, Nicolas
Kammerbauer, Fabian
Masciovecchio, Claudio
Mincigrucci, Riccardo
Nelson, Keith A.
Paltanin, Ettore
Pelli-Cresi, Jacopo Stefano
Polewczyk, Vincent
Ksenzov, Dmitriy
Bencivenga, Filippo
author_facet Maznev, Alexei A.
Lee, Wonseok
Cushing, Scott K.
De Angelis, Dario
Fainozzi, Danny
Foglia, Laura
Gutt, Christian
Jaouen, Nicolas
Kammerbauer, Fabian
Masciovecchio, Claudio
Mincigrucci, Riccardo
Nelson, Keith A.
Paltanin, Ettore
Pelli-Cresi, Jacopo Stefano
Polewczyk, Vincent
Ksenzov, Dmitriy
Bencivenga, Filippo
contents Self-diffraction is a non-collinear four-wave mixing technique well-known in optics. We explore self-diffraction in the extreme ultraviolet (EUV) range, taking advantage of intense femtosecond EUV pulses produced by a free electron laser. Two pulses are crossed in a thin cobalt film and their interference results in a spatially periodic electronic excitation. The diffraction of one of the same pulses by the associated refractive index modulation is measured as a function of the EUV wavelength. A sharp peak in the self-diffraction efficiency is observed at the M$_{2,3}$ absorption edge of cobalt at 59 eV and a fine structure is found above the edge. The results are compared with a theoretical model assuming that the excitation results in an increase of the electronic temperature. EUV self-diffraction offers a potentially useful spectroscopy tool and will be instrumental in studying coherent effects in the EUV range.
format Preprint
id arxiv_https___arxiv_org_abs_2505_07168
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Resonant Self-Diffraction of Femtosecond Extreme Ultraviolet Pulses in Cobalt
Maznev, Alexei A.
Lee, Wonseok
Cushing, Scott K.
De Angelis, Dario
Fainozzi, Danny
Foglia, Laura
Gutt, Christian
Jaouen, Nicolas
Kammerbauer, Fabian
Masciovecchio, Claudio
Mincigrucci, Riccardo
Nelson, Keith A.
Paltanin, Ettore
Pelli-Cresi, Jacopo Stefano
Polewczyk, Vincent
Ksenzov, Dmitriy
Bencivenga, Filippo
Optics
Materials Science
Self-diffraction is a non-collinear four-wave mixing technique well-known in optics. We explore self-diffraction in the extreme ultraviolet (EUV) range, taking advantage of intense femtosecond EUV pulses produced by a free electron laser. Two pulses are crossed in a thin cobalt film and their interference results in a spatially periodic electronic excitation. The diffraction of one of the same pulses by the associated refractive index modulation is measured as a function of the EUV wavelength. A sharp peak in the self-diffraction efficiency is observed at the M$_{2,3}$ absorption edge of cobalt at 59 eV and a fine structure is found above the edge. The results are compared with a theoretical model assuming that the excitation results in an increase of the electronic temperature. EUV self-diffraction offers a potentially useful spectroscopy tool and will be instrumental in studying coherent effects in the EUV range.
title Resonant Self-Diffraction of Femtosecond Extreme Ultraviolet Pulses in Cobalt
topic Optics
Materials Science
url https://arxiv.org/abs/2505.07168