Current-induced Nonequilibrium Phase Transition Accompanied by Giant Gap Reduction in Vanadium Dioxide

Fuente: arXiv
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Autori principali: Nakano, Akitoshi, Imaizumi, Masato, Terasaki, Ichiro
Natura: Preprint
Pubblicazione: 2025
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author Nakano, Akitoshi
Imaizumi, Masato
Terasaki, Ichiro
author_facet Nakano, Akitoshi
Imaizumi, Masato
Terasaki, Ichiro
contents We investigated nonlinear conduction in bulk single crystals of VO2 with precise temperature control. Two distinct nonequilibrium phenomena were identified: a gradual reduction of the charge gap and a current-induced insulator-metal transition. The electric field required to drive the nonlinear conduction is two to three orders of magnitude smaller than that reported for VO2 thin films or nanobeams, strongly indicating an intrinsic electronic origin rather than a temperature increase due to self heating. Notably, our results suggest that the application of a steady current to the frozen insulating state can induce a nonequilibrium steady-state metallic phase -- effectively melting the electronic ice. This highlights a novel route to controlling electronic states via nonthermal, current-driven mechanisms.
format Preprint
id arxiv_https___arxiv_org_abs_2505_07307
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Current-induced Nonequilibrium Phase Transition Accompanied by Giant Gap Reduction in Vanadium Dioxide
Nakano, Akitoshi
Imaizumi, Masato
Terasaki, Ichiro
Strongly Correlated Electrons
We investigated nonlinear conduction in bulk single crystals of VO2 with precise temperature control. Two distinct nonequilibrium phenomena were identified: a gradual reduction of the charge gap and a current-induced insulator-metal transition. The electric field required to drive the nonlinear conduction is two to three orders of magnitude smaller than that reported for VO2 thin films or nanobeams, strongly indicating an intrinsic electronic origin rather than a temperature increase due to self heating. Notably, our results suggest that the application of a steady current to the frozen insulating state can induce a nonequilibrium steady-state metallic phase -- effectively melting the electronic ice. This highlights a novel route to controlling electronic states via nonthermal, current-driven mechanisms.
title Current-induced Nonequilibrium Phase Transition Accompanied by Giant Gap Reduction in Vanadium Dioxide
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2505.07307