Experimental Observation of Short-Range Magnetic Correlations in Amorphous Nb$_2$O$_5$ and Ta$_2$O$_5$ Thin Films

Fuente: arXiv
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Hauptverfasser: Krasnikova, Y. V., Murthy, A. A., Bafia, D., Crisa, F., Clairmont, A., Sung, Z., Lee, J., Cano, A., Shinde, M., van Zanten, D. M. T., Bal, M., Romanenko, A., Grassellino, A., Dhundhwal, R., Fuchs, D., Reisinger, T., Pop, I. M., Suter, A., Prokscha, T., Salman, Z.
Format: Preprint
Veröffentlicht: 2025
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author Krasnikova, Y. V.
Murthy, A. A.
Bafia, D.
Crisa, F.
Clairmont, A.
Sung, Z.
Lee, J.
Cano, A.
Shinde, M.
van Zanten, D. M. T.
Bal, M.
Romanenko, A.
Grassellino, A.
Dhundhwal, R.
Fuchs, D.
Reisinger, T.
Pop, I. M.
Suter, A.
Prokscha, T.
Salman, Z.
author_facet Krasnikova, Y. V.
Murthy, A. A.
Bafia, D.
Crisa, F.
Clairmont, A.
Sung, Z.
Lee, J.
Cano, A.
Shinde, M.
van Zanten, D. M. T.
Bal, M.
Romanenko, A.
Grassellino, A.
Dhundhwal, R.
Fuchs, D.
Reisinger, T.
Pop, I. M.
Suter, A.
Prokscha, T.
Salman, Z.
contents We use muon spin rotation/relaxation/resonance ($μ$SR) to investigate the magnetic properties of niobium pentoxide (Nb$_2$O$_5$) and tantalum pentoxide (Ta$_2$O$_5$) thin films. In both oxides, we observe a magnetic response at the lowest available temperature of 2.8 K. This response appears to be structurally dependent: thermally oxidized Ta$_2$O$_5$ with low crystallinity demonstrates suppressed magnetism, while fully amorphous Ta$_2$O$_5$ demonstrates local static magnetism. In contrast, amorphous Nb$_2$O$_5$ is dominated by magnetic fluctuations and is strongly magnetically disordered compared to Ta$_2$O$_5$. Our results suggest that these fundamental differences in the magnetism of Ta and Nb oxides could explain the performance limitations in superconducting qubits and resonators.
format Preprint
id arxiv_https___arxiv_org_abs_2505_07957
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Experimental Observation of Short-Range Magnetic Correlations in Amorphous Nb$_2$O$_5$ and Ta$_2$O$_5$ Thin Films
Krasnikova, Y. V.
Murthy, A. A.
Bafia, D.
Crisa, F.
Clairmont, A.
Sung, Z.
Lee, J.
Cano, A.
Shinde, M.
van Zanten, D. M. T.
Bal, M.
Romanenko, A.
Grassellino, A.
Dhundhwal, R.
Fuchs, D.
Reisinger, T.
Pop, I. M.
Suter, A.
Prokscha, T.
Salman, Z.
Other Condensed Matter
Quantum Physics
We use muon spin rotation/relaxation/resonance ($μ$SR) to investigate the magnetic properties of niobium pentoxide (Nb$_2$O$_5$) and tantalum pentoxide (Ta$_2$O$_5$) thin films. In both oxides, we observe a magnetic response at the lowest available temperature of 2.8 K. This response appears to be structurally dependent: thermally oxidized Ta$_2$O$_5$ with low crystallinity demonstrates suppressed magnetism, while fully amorphous Ta$_2$O$_5$ demonstrates local static magnetism. In contrast, amorphous Nb$_2$O$_5$ is dominated by magnetic fluctuations and is strongly magnetically disordered compared to Ta$_2$O$_5$. Our results suggest that these fundamental differences in the magnetism of Ta and Nb oxides could explain the performance limitations in superconducting qubits and resonators.
title Experimental Observation of Short-Range Magnetic Correlations in Amorphous Nb$_2$O$_5$ and Ta$_2$O$_5$ Thin Films
topic Other Condensed Matter
Quantum Physics
url https://arxiv.org/abs/2505.07957