Solute mixing in porous media with dispersion and buoyancy

Fuente: arXiv
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Autori principali: De Paoli, Marco, Yerragolam, Guru Sreevanshu, Verzicco, Roberto, Lohse, Detlef
Natura: Preprint
Pubblicazione: 2025
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author De Paoli, Marco
Yerragolam, Guru Sreevanshu
Verzicco, Roberto
Lohse, Detlef
author_facet De Paoli, Marco
Yerragolam, Guru Sreevanshu
Verzicco, Roberto
Lohse, Detlef
contents We analyse the process of convective mixing in two-dimensional, homogeneous and isotropic porous media with dispersion. We considered a Rayleigh-Taylor instability in which the presence of a solute produces density differences driving the flow. The effect of dispersion is modelled using an anisotropic Fickian dispersion tensor (Bear, J. Geophys. Res. 1961). In addition to molecular diffusion ($D_m^*$), the solute is redistributed by an additional spreading, in longitudinal and transverse flow directions, which is quantified by the coefficients $D_l^*$ and $D_t^*$, respectively, and it is produced by the presence of the pores. The flow is controlled by three dimensionless parameters: the Rayleigh-Darcy number $Ra$, defining the relative strength of convection and diffusion, and the dispersion parameters $r=D_l^*/D_t^*$ and $Δ=D_m^*/D_t^*$. With the aid of numerical Darcy simulations, we investigate the mixing dynamics without and with dispersion. We find that in absence of dispersion ($Δ\to\infty$) the dynamics is self-similar and independent of $Ra$, and the flow evolves following several regimes, which we analyse. Then we analyse the effect of dispersion on the flow evolution for a fixed value of the Rayleigh-Darcy number ($Ra=10^4$). A detailed analysis of the molecular and dispersive components of the mean scalar dissipation reveals a complex interplay between flow structures and solute mixing. The proposed theoretical framework, in combination with pore-scale simulations and bead packs experiments, can be used to validate and improve current dispersion models to obtain more reliable estimates of solute transport and spreading in buoyancy-driven subsurface flows.
format Preprint
id arxiv_https___arxiv_org_abs_2505_11005
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Solute mixing in porous media with dispersion and buoyancy
De Paoli, Marco
Yerragolam, Guru Sreevanshu
Verzicco, Roberto
Lohse, Detlef
Fluid Dynamics
Geophysics
We analyse the process of convective mixing in two-dimensional, homogeneous and isotropic porous media with dispersion. We considered a Rayleigh-Taylor instability in which the presence of a solute produces density differences driving the flow. The effect of dispersion is modelled using an anisotropic Fickian dispersion tensor (Bear, J. Geophys. Res. 1961). In addition to molecular diffusion ($D_m^*$), the solute is redistributed by an additional spreading, in longitudinal and transverse flow directions, which is quantified by the coefficients $D_l^*$ and $D_t^*$, respectively, and it is produced by the presence of the pores. The flow is controlled by three dimensionless parameters: the Rayleigh-Darcy number $Ra$, defining the relative strength of convection and diffusion, and the dispersion parameters $r=D_l^*/D_t^*$ and $Δ=D_m^*/D_t^*$. With the aid of numerical Darcy simulations, we investigate the mixing dynamics without and with dispersion. We find that in absence of dispersion ($Δ\to\infty$) the dynamics is self-similar and independent of $Ra$, and the flow evolves following several regimes, which we analyse. Then we analyse the effect of dispersion on the flow evolution for a fixed value of the Rayleigh-Darcy number ($Ra=10^4$). A detailed analysis of the molecular and dispersive components of the mean scalar dissipation reveals a complex interplay between flow structures and solute mixing. The proposed theoretical framework, in combination with pore-scale simulations and bead packs experiments, can be used to validate and improve current dispersion models to obtain more reliable estimates of solute transport and spreading in buoyancy-driven subsurface flows.
title Solute mixing in porous media with dispersion and buoyancy
topic Fluid Dynamics
Geophysics
url https://arxiv.org/abs/2505.11005