Electronic mobility, doping, and defects in epitaxial $\mathrm{BaZrS_3}$ chalcogenide perovskite thin films

Fuente: arXiv
Guardado en:
Detalles Bibliográficos
Autores principales: Van Sambeek, Jack, Dong, Jessica, Ievlev, Anton V., Cai, Tao, Sadeghi, Ida, Jaramillo, Rafael
Formato: Preprint
Publicado: 2025
Materias:
Acceso en línea:
Etiquetas: Agregar Etiqueta
Sin Etiquetas, Sea el primero en etiquetar este registro!
_version_ 1866910982008209408
author Van Sambeek, Jack
Dong, Jessica
Ievlev, Anton V.
Cai, Tao
Sadeghi, Ida
Jaramillo, Rafael
author_facet Van Sambeek, Jack
Dong, Jessica
Ievlev, Anton V.
Cai, Tao
Sadeghi, Ida
Jaramillo, Rafael
contents We present the electronic transport properties of $\mathrm{BaZrS_3}$ (BZS) thin films grown epitaxially by gas-source molecular beam epitaxy (MBE). We observe n-type behavior in all samples, with carrier concentration ranging from $4 \times 10^{18}$ to $4 \times 10^{20} \mathrm{cm^{-3}}$ at room temperature (RT). We observe a champion RT Hall mobility of 11.1 $\mathrm{cm^2V^{-1}s^{-1}}$, which is competitive with established thin-film photovoltaic (PV) absorbers. Temperature-dependent Hall mobility data show that phonon scattering dominates at room temperature, in agreement with computational predictions. X-ray diffraction data illustrate a correlation between mobility and stacking fault concentration, illustrating how microstructure can affect transport. Despite the well-established environmental stability of chalcogenide perovskites, we observe significant changes to electronic properties as a function of storage time in ambient conditions. With the help of secondary-ion mass-spectrometry (SIMS) measurements, we propose and support a defect mechanism that explains this behavior: as-grown films have a high concentration of sulfur vacancies that are shallow donors ($\mathrm{V_S^\bullet}$ or $\mathrm{V_S^{\bullet \bullet}}$), which are converted into neutral oxygen defects ($\mathrm{O_S^\times}$) upon air exposure. We discuss the relevance of this defect mechanism within the larger context of chalcogenide perovskite research, and we identify means to stabilize the electronic properties.
format Preprint
id arxiv_https___arxiv_org_abs_2505_16016
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Electronic mobility, doping, and defects in epitaxial $\mathrm{BaZrS_3}$ chalcogenide perovskite thin films
Van Sambeek, Jack
Dong, Jessica
Ievlev, Anton V.
Cai, Tao
Sadeghi, Ida
Jaramillo, Rafael
Materials Science
We present the electronic transport properties of $\mathrm{BaZrS_3}$ (BZS) thin films grown epitaxially by gas-source molecular beam epitaxy (MBE). We observe n-type behavior in all samples, with carrier concentration ranging from $4 \times 10^{18}$ to $4 \times 10^{20} \mathrm{cm^{-3}}$ at room temperature (RT). We observe a champion RT Hall mobility of 11.1 $\mathrm{cm^2V^{-1}s^{-1}}$, which is competitive with established thin-film photovoltaic (PV) absorbers. Temperature-dependent Hall mobility data show that phonon scattering dominates at room temperature, in agreement with computational predictions. X-ray diffraction data illustrate a correlation between mobility and stacking fault concentration, illustrating how microstructure can affect transport. Despite the well-established environmental stability of chalcogenide perovskites, we observe significant changes to electronic properties as a function of storage time in ambient conditions. With the help of secondary-ion mass-spectrometry (SIMS) measurements, we propose and support a defect mechanism that explains this behavior: as-grown films have a high concentration of sulfur vacancies that are shallow donors ($\mathrm{V_S^\bullet}$ or $\mathrm{V_S^{\bullet \bullet}}$), which are converted into neutral oxygen defects ($\mathrm{O_S^\times}$) upon air exposure. We discuss the relevance of this defect mechanism within the larger context of chalcogenide perovskite research, and we identify means to stabilize the electronic properties.
title Electronic mobility, doping, and defects in epitaxial $\mathrm{BaZrS_3}$ chalcogenide perovskite thin films
topic Materials Science
url https://arxiv.org/abs/2505.16016