Spin adaptation of the cumulant expansions of reduced density matrices

Fuente: arXiv
Saved in:
Bibliographic Details
Main Authors: Liebert, Julia, Schilling, Christian, Mazziotti, David A.
Format: Preprint
Published: 2025
Subjects:
Online Access:
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1866912677606981632
author Liebert, Julia
Schilling, Christian
Mazziotti, David A.
author_facet Liebert, Julia
Schilling, Christian
Mazziotti, David A.
contents We develop a systematic framework for the spin adaptation of the cumulants of p-particle reduced density matrices (RDMs), with explicit constructions for p = 1 to 3. These spin-adapted cumulants enable rigorous treatment of both S_z and S^2 symmetries in quantum systems, providing a foundation for spin-resolved electronic structure methods. We show that complete spin adaptation -- referred to as complete S-representability -- can be enforced by constraining the variances of S_z and S^2, which require the 2-RDM and 4-RDM, respectively. Importantly, the cumulants of RDMs scale linearly with system size -- size-extensive -- making them a natural object for incorporating spin symmetries in scalable electronic structure theories. The developed formalism is applicable to density-based methods (DFT), one-particle RDM functional theories (RDMFT), and two-particle RDM methods. We further extend the approach to spin-orbit-coupled systems via total angular momentum adaptation. Beyond spin, the framework enables the adaptation of RDM theories to additional symmetries through the construction of suitable irreducible tensor operators.
format Preprint
id arxiv_https___arxiv_org_abs_2505_16989
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Spin adaptation of the cumulant expansions of reduced density matrices
Liebert, Julia
Schilling, Christian
Mazziotti, David A.
Chemical Physics
Computational Physics
Quantum Physics
We develop a systematic framework for the spin adaptation of the cumulants of p-particle reduced density matrices (RDMs), with explicit constructions for p = 1 to 3. These spin-adapted cumulants enable rigorous treatment of both S_z and S^2 symmetries in quantum systems, providing a foundation for spin-resolved electronic structure methods. We show that complete spin adaptation -- referred to as complete S-representability -- can be enforced by constraining the variances of S_z and S^2, which require the 2-RDM and 4-RDM, respectively. Importantly, the cumulants of RDMs scale linearly with system size -- size-extensive -- making them a natural object for incorporating spin symmetries in scalable electronic structure theories. The developed formalism is applicable to density-based methods (DFT), one-particle RDM functional theories (RDMFT), and two-particle RDM methods. We further extend the approach to spin-orbit-coupled systems via total angular momentum adaptation. Beyond spin, the framework enables the adaptation of RDM theories to additional symmetries through the construction of suitable irreducible tensor operators.
title Spin adaptation of the cumulant expansions of reduced density matrices
topic Chemical Physics
Computational Physics
Quantum Physics
url https://arxiv.org/abs/2505.16989