Acceleration of enzymatic reaction-diffusion kinetics by intermediate state

Fuente: arXiv
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Autores principales: Fukuda, Akihiro, Nakayama, Yohei, Toyabe, Shoichi
Formato: Preprint
Publicado: 2025
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author Fukuda, Akihiro
Nakayama, Yohei
Toyabe, Shoichi
author_facet Fukuda, Akihiro
Nakayama, Yohei
Toyabe, Shoichi
contents Biological molecular motors are high-performance nanomachines that convert chemical energy into mechanical motion via chemomechanical coupling. Their reaction cycles typically comprise a series of intermediate chemical states between the initial and final primary states. However, the influence of these intermediate states on motor performance has not yet been fully explored. In this study, we investigate the impact of intermediate states on the motor kinetics using a reaction-diffusion model. In most cases, the intermediate states accelerate the motor by lowering the effective barrier height. This acceleration is particularly pronounced when an external load is applied to the motor, implying the practical importance of the intermediate states. The intermediate states can also slow down the reaction in some cases, such as the slow reaction limit with asymmetric kinetics. Our findings provide practical insights into the design principles behind the high performance of biological molecular motors, as well as the development of efficient artificial molecular motors.
format Preprint
id arxiv_https___arxiv_org_abs_2505_17130
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Acceleration of enzymatic reaction-diffusion kinetics by intermediate state
Fukuda, Akihiro
Nakayama, Yohei
Toyabe, Shoichi
Biological Physics
Statistical Mechanics
Biological molecular motors are high-performance nanomachines that convert chemical energy into mechanical motion via chemomechanical coupling. Their reaction cycles typically comprise a series of intermediate chemical states between the initial and final primary states. However, the influence of these intermediate states on motor performance has not yet been fully explored. In this study, we investigate the impact of intermediate states on the motor kinetics using a reaction-diffusion model. In most cases, the intermediate states accelerate the motor by lowering the effective barrier height. This acceleration is particularly pronounced when an external load is applied to the motor, implying the practical importance of the intermediate states. The intermediate states can also slow down the reaction in some cases, such as the slow reaction limit with asymmetric kinetics. Our findings provide practical insights into the design principles behind the high performance of biological molecular motors, as well as the development of efficient artificial molecular motors.
title Acceleration of enzymatic reaction-diffusion kinetics by intermediate state
topic Biological Physics
Statistical Mechanics
url https://arxiv.org/abs/2505.17130