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Bibliographische Detailangaben
Hauptverfasser: Weiss, Leah R., Smith, Grant T., Murphy, Ryan A., Golesorkhi, Bahman, Méndez, José A. Méndez, Patel, Priya, Niklas, Jens, Poluektov, Oleg G., Long, Jeffrey R., Awschalom, David D.
Format: Preprint
Veröffentlicht: 2025
Schlagworte:
Online-Zugang:https://arxiv.org/abs/2505.17195
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Inhaltsangabe:
  • Optically addressable electronic spins in polyatomic molecules are a promising platform for quantum information science with the potential to enable scalable qubit design and integration through atomistic tunability and nanoscale localization. However, optical state- and site-selection are an open challenge. Here we introduce an organo-erbium spin qubit in which narrow (MHz-scale) optical and spin transitions couple to provide high-resolution access to spin degrees of freedom with telecommunications frequency light. This spin-photon interface enables demonstration of optical spin polarization and readout that distinguishes between spin states and magnetically inequivalent sites in a molecular crystal. Operation at frequencies compatible with mature photonic and microwave devices opens a path for engineering scalable, integrated molecular spin-optical quantum technologies.