Room-temperature spin-lifetime anisotropy exceeding 60 in bilayer graphene spin valves proximity coupled to WSe$_2$

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Main Authors: Bisswanger, Timo, Schmidt, Anne, Volmer, Frank, Stampfer, Christoph, Beschoten, Bernd
Format: Preprint
Published: 2025
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author Bisswanger, Timo
Schmidt, Anne
Volmer, Frank
Stampfer, Christoph
Beschoten, Bernd
author_facet Bisswanger, Timo
Schmidt, Anne
Volmer, Frank
Stampfer, Christoph
Beschoten, Bernd
contents A spin lifetime anisotropy between in-plane and out-of-plane spins in bilayer graphene (BLG) can be achieved by spin-orbit proximity coupling of graphene to transition metal dichalcogenides. This coupling reduces the in-plane spin lifetime due to proximity-induced spin scattering, while the out-of-plane spin lifetime remains largely unaffected. We show that at room temperature spin lifetime anisotropy exceeds 60 in a bilayer graphene lateral spin valve proximity coupled to WSe$_2$. The out-of-plane spin lifetime of about 250 ps closely matches that of a BLG reference region not in contact with WSe$_2$. In contrast, the estimated in-plane spin lifetime of less than 4 ps leads to a complete suppression of the in-plane spin signal at the ferromagnetic Co/MgO spin detector. The proximity coupling of WSe$_2$ to BLG is particularly promising, as it does not compromise the charge carrier mobility within the graphene channel.
format Preprint
id arxiv_https___arxiv_org_abs_2505_18990
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Room-temperature spin-lifetime anisotropy exceeding 60 in bilayer graphene spin valves proximity coupled to WSe$_2$
Bisswanger, Timo
Schmidt, Anne
Volmer, Frank
Stampfer, Christoph
Beschoten, Bernd
Mesoscale and Nanoscale Physics
Materials Science
A spin lifetime anisotropy between in-plane and out-of-plane spins in bilayer graphene (BLG) can be achieved by spin-orbit proximity coupling of graphene to transition metal dichalcogenides. This coupling reduces the in-plane spin lifetime due to proximity-induced spin scattering, while the out-of-plane spin lifetime remains largely unaffected. We show that at room temperature spin lifetime anisotropy exceeds 60 in a bilayer graphene lateral spin valve proximity coupled to WSe$_2$. The out-of-plane spin lifetime of about 250 ps closely matches that of a BLG reference region not in contact with WSe$_2$. In contrast, the estimated in-plane spin lifetime of less than 4 ps leads to a complete suppression of the in-plane spin signal at the ferromagnetic Co/MgO spin detector. The proximity coupling of WSe$_2$ to BLG is particularly promising, as it does not compromise the charge carrier mobility within the graphene channel.
title Room-temperature spin-lifetime anisotropy exceeding 60 in bilayer graphene spin valves proximity coupled to WSe$_2$
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2505.18990