Strain-induced magnetic damping anomaly in La$_{1-x}$Sr$_{x}$MnO$_{3}$ ($x=0.3$-$0.5$) thin films

Fuente: arXiv
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Autores principales: Arakawa, Ryotaro, Komori, Sachio, Taniyama, Tomoyasu
Formato: Preprint
Publicado: 2025
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author Arakawa, Ryotaro
Komori, Sachio
Taniyama, Tomoyasu
author_facet Arakawa, Ryotaro
Komori, Sachio
Taniyama, Tomoyasu
contents Magnetic properties of La$_{1-x}$Sr$_x$MnO$_{3}$ (LSMO) are highly sensitive to various factors such as the Sr doping level $x$, lattice strain, and oxygen stoichiometry due to the strongly correlated nature of $3d$ electrons. For the development of energy-efficient spintronic devices with ultra-low magnetic damping of LSMO, a thorough understanding of its complex magnetization dynamics is of great importance. In this work, we have measured ferromagnetic resonance of LSMO thin films on Nb-doped SrTiO$_3$ (Nb-STO) substrates over a wide temperature and frequency range and observed an anomalous increase in the Gilbert damping constant and a decrease in the effective saturation magnetization at temperatures below 100 K. The anomalies become more pronounced as the LSMO thickness decreases while they are not observed for LSMO on (LaAlO$_3$)$_{0.3}$(Sr$_2$TaAlO$_6$)$_{0.7}$ substrates with relatively small epitaxial strain. The results suggest that the epitaxial strain-induced magnetically dead layer at the LSMO/Nb-STO interface acts as a spin sink and leads to the anomalies in the magnetization dynamics.
format Preprint
id arxiv_https___arxiv_org_abs_2505_19005
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Strain-induced magnetic damping anomaly in La$_{1-x}$Sr$_{x}$MnO$_{3}$ ($x=0.3$-$0.5$) thin films
Arakawa, Ryotaro
Komori, Sachio
Taniyama, Tomoyasu
Mesoscale and Nanoscale Physics
Materials Science
Strongly Correlated Electrons
Magnetic properties of La$_{1-x}$Sr$_x$MnO$_{3}$ (LSMO) are highly sensitive to various factors such as the Sr doping level $x$, lattice strain, and oxygen stoichiometry due to the strongly correlated nature of $3d$ electrons. For the development of energy-efficient spintronic devices with ultra-low magnetic damping of LSMO, a thorough understanding of its complex magnetization dynamics is of great importance. In this work, we have measured ferromagnetic resonance of LSMO thin films on Nb-doped SrTiO$_3$ (Nb-STO) substrates over a wide temperature and frequency range and observed an anomalous increase in the Gilbert damping constant and a decrease in the effective saturation magnetization at temperatures below 100 K. The anomalies become more pronounced as the LSMO thickness decreases while they are not observed for LSMO on (LaAlO$_3$)$_{0.3}$(Sr$_2$TaAlO$_6$)$_{0.7}$ substrates with relatively small epitaxial strain. The results suggest that the epitaxial strain-induced magnetically dead layer at the LSMO/Nb-STO interface acts as a spin sink and leads to the anomalies in the magnetization dynamics.
title Strain-induced magnetic damping anomaly in La$_{1-x}$Sr$_{x}$MnO$_{3}$ ($x=0.3$-$0.5$) thin films
topic Mesoscale and Nanoscale Physics
Materials Science
Strongly Correlated Electrons
url https://arxiv.org/abs/2505.19005