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Main Authors: Jeon, Kun-Rok, Kim, Jae-Keun, Yoon, Jiho, Jeon, Jae-Chun, Han, Hyeon, Cottet, Audrey, Kontos, Takis, Parkin, Stuart S. P.
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2505.20598
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author Jeon, Kun-Rok
Kim, Jae-Keun
Yoon, Jiho
Jeon, Jae-Chun
Han, Hyeon
Cottet, Audrey
Kontos, Takis
Parkin, Stuart S. P.
author_facet Jeon, Kun-Rok
Kim, Jae-Keun
Yoon, Jiho
Jeon, Jae-Chun
Han, Hyeon
Cottet, Audrey
Kontos, Takis
Parkin, Stuart S. P.
contents The recent realization of zero-field, polarity-reversible supercurrent rectification in proximity-magnetized Rashba-type Pt Josephson junctions (JJs) enables the development of superconducting logic circuits and cryogenic memory applications. Here, we demonstrate a non-volatile anomalous phase shift ϕ_0 directly probed via superconducting quantum interferometry, providing phase-sensitive evidence of spontaneous time-reversal symmetry breaking in these Rashba-type systems. By replacing the Pt barrier with 5d or 4d element layers exhibiting different (para-)magnetic susceptibilities, spin-orbit coupling strengths, and electronic band structures, we elucidate the role of proximity effects in governing zero-field diode behavior. Ta (W) JJs exhibit zero-field diode efficiencies of ~17% (~5%) at 2 K, which are slightly (significantly) lower than those of Pt JJs. Notably, the diode polarity in Ta and W JJs is reversed relative to Pt JJs. Combined with the large zero-field diode efficiency (~15% at 2 K) observed in highly magnetic-susceptible Pd JJs, these results show that non-volatile ϕ_0 and, consequently, zero-field diode performance can be tuned through proximity engineering of interfacial magnetic ordering and Rashba spin-orbit interaction.
format Preprint
id arxiv_https___arxiv_org_abs_2505_20598
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Interferometric evidence of non-volatile anomalous phase shifts in exchange-spin-split Josephson supercurrent diodes
Jeon, Kun-Rok
Kim, Jae-Keun
Yoon, Jiho
Jeon, Jae-Chun
Han, Hyeon
Cottet, Audrey
Kontos, Takis
Parkin, Stuart S. P.
Superconductivity
The recent realization of zero-field, polarity-reversible supercurrent rectification in proximity-magnetized Rashba-type Pt Josephson junctions (JJs) enables the development of superconducting logic circuits and cryogenic memory applications. Here, we demonstrate a non-volatile anomalous phase shift ϕ_0 directly probed via superconducting quantum interferometry, providing phase-sensitive evidence of spontaneous time-reversal symmetry breaking in these Rashba-type systems. By replacing the Pt barrier with 5d or 4d element layers exhibiting different (para-)magnetic susceptibilities, spin-orbit coupling strengths, and electronic band structures, we elucidate the role of proximity effects in governing zero-field diode behavior. Ta (W) JJs exhibit zero-field diode efficiencies of ~17% (~5%) at 2 K, which are slightly (significantly) lower than those of Pt JJs. Notably, the diode polarity in Ta and W JJs is reversed relative to Pt JJs. Combined with the large zero-field diode efficiency (~15% at 2 K) observed in highly magnetic-susceptible Pd JJs, these results show that non-volatile ϕ_0 and, consequently, zero-field diode performance can be tuned through proximity engineering of interfacial magnetic ordering and Rashba spin-orbit interaction.
title Interferometric evidence of non-volatile anomalous phase shifts in exchange-spin-split Josephson supercurrent diodes
topic Superconductivity
url https://arxiv.org/abs/2505.20598