Unconventional Orbital Magnetism in Graphene-based Fractional Chern Insulators

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Main Authors: Xie, Jian, Zhang, Zaizhe, Chen, Xi, Kwan, Yves H., Huo, Zihao, Herzog-Arbeitman, Jonah, Guo, Liangliang, Watanabe, Kenji, Taniguchi, Takashi, Liu, Kaihui, Xie, X. C., Bernevig, B. Andrei, Song, Zhi-Da, Lu, Xiaobo
Format: Preprint
Published: 2025
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author Xie, Jian
Zhang, Zaizhe
Chen, Xi
Kwan, Yves H.
Huo, Zihao
Herzog-Arbeitman, Jonah
Guo, Liangliang
Watanabe, Kenji
Taniguchi, Takashi
Liu, Kaihui
Xie, X. C.
Bernevig, B. Andrei
Song, Zhi-Da
Lu, Xiaobo
author_facet Xie, Jian
Zhang, Zaizhe
Chen, Xi
Kwan, Yves H.
Huo, Zihao
Herzog-Arbeitman, Jonah
Guo, Liangliang
Watanabe, Kenji
Taniguchi, Takashi
Liu, Kaihui
Xie, X. C.
Bernevig, B. Andrei
Song, Zhi-Da
Lu, Xiaobo
contents Orbital magnetism in graphene originates from correlation-driven spontaneous valley symmetry breaking1-7. It can lead to various anomalous transport phenomena such as integer and fractional quantum anomalous Hall effects8-11. In general, the in-plane magnetic field B|| primarily couples to the spin degrees of freedom in graphene and has long been presumed to have a negligible effect on orbital magnetism due to the ultra-weak spin-orbit coupling12-18. In this work, we report multiple unconventional orbital magnetic phenomena that are highly sensitive to the B|| field in graphene/hBN superlattices hosting both integer and fractional Chern insulators (FCIs). We observed chirality-switching behaviors of the Chern insulator at moiré filling factor ν = 1 under a finite B_par, demonstrating that both the C = +-1 states are permissible ground states at zero perpendicular magnetic field B_per. For the FCI at ν = 2/3, we observed topological phase transitions between two states characterized by Hall resistivity \r{ho}xy = +-3h/2e2 under both B_per and B_par fields. In-plane B|| field can effectively suppress the FCI state at zero B_per field and enhance the FCI state with the opposite chirality, as resolved in Landau fan diagrams. Moreover, we observed rich phase transitions at 1 < ν < 2, accompanied by intervalley coherence and anomalous Hall effects (AHE) that can be triggered by sweeping either B_per or B_par. Our work has unveiled new properties of orbital magnetism, providing a new knob for engineering various AHE in graphene.
format Preprint
id arxiv_https___arxiv_org_abs_2506_01485
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Unconventional Orbital Magnetism in Graphene-based Fractional Chern Insulators
Xie, Jian
Zhang, Zaizhe
Chen, Xi
Kwan, Yves H.
Huo, Zihao
Herzog-Arbeitman, Jonah
Guo, Liangliang
Watanabe, Kenji
Taniguchi, Takashi
Liu, Kaihui
Xie, X. C.
Bernevig, B. Andrei
Song, Zhi-Da
Lu, Xiaobo
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Orbital magnetism in graphene originates from correlation-driven spontaneous valley symmetry breaking1-7. It can lead to various anomalous transport phenomena such as integer and fractional quantum anomalous Hall effects8-11. In general, the in-plane magnetic field B|| primarily couples to the spin degrees of freedom in graphene and has long been presumed to have a negligible effect on orbital magnetism due to the ultra-weak spin-orbit coupling12-18. In this work, we report multiple unconventional orbital magnetic phenomena that are highly sensitive to the B|| field in graphene/hBN superlattices hosting both integer and fractional Chern insulators (FCIs). We observed chirality-switching behaviors of the Chern insulator at moiré filling factor ν = 1 under a finite B_par, demonstrating that both the C = +-1 states are permissible ground states at zero perpendicular magnetic field B_per. For the FCI at ν = 2/3, we observed topological phase transitions between two states characterized by Hall resistivity \r{ho}xy = +-3h/2e2 under both B_per and B_par fields. In-plane B|| field can effectively suppress the FCI state at zero B_per field and enhance the FCI state with the opposite chirality, as resolved in Landau fan diagrams. Moreover, we observed rich phase transitions at 1 < ν < 2, accompanied by intervalley coherence and anomalous Hall effects (AHE) that can be triggered by sweeping either B_per or B_par. Our work has unveiled new properties of orbital magnetism, providing a new knob for engineering various AHE in graphene.
title Unconventional Orbital Magnetism in Graphene-based Fractional Chern Insulators
topic Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
url https://arxiv.org/abs/2506.01485