Electrically-induced resonance shifts of whispering gallery resonators made of barium magnesium fluoride

Fuente: arXiv
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Main Authors: Mrokon, Alexander, Kraft, Heike, Shin, Dongsung, Tanaka, Hiroki, Herr, Simon J., Buse, Karsten, Breunig, Ingo
Format: Preprint
Published: 2025
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author Mrokon, Alexander
Kraft, Heike
Shin, Dongsung
Tanaka, Hiroki
Herr, Simon J.
Buse, Karsten
Breunig, Ingo
author_facet Mrokon, Alexander
Kraft, Heike
Shin, Dongsung
Tanaka, Hiroki
Herr, Simon J.
Buse, Karsten
Breunig, Ingo
contents Barium magnesium fluoride (BMF) is a ferroelectric crystal with a transparency range far beyond the one of other optical materials. In particular, its low loss in the deep ultraviolet makes this material an unique candidate for frequency conversion in this spectral range. Due to its relatively weak second-order nonlinearity, a resonant configuration such as an optical whispering gallery would be beneficial. We show that femtosecond-laser based material processing enables the reliable fabrication of BMF whispering gallery resonators with quality factors beyond $10^7$. Their resonance frequencies can be shifted linearly by applying electric fields between the $+c$ and $-c$ faces of the crystal. The slope of the shift is $-0.8$~MHz/(V/mm). It seems that the origin of this shift is piezoelectricity, while the electro-optic effect is negligible. Our results pave the way for millimeter-sized frequency converters in the deep ultraviolet. Furthermore, they indicate that a careful determination of fundamental material properties is still necessary.
format Preprint
id arxiv_https___arxiv_org_abs_2506_03873
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Electrically-induced resonance shifts of whispering gallery resonators made of barium magnesium fluoride
Mrokon, Alexander
Kraft, Heike
Shin, Dongsung
Tanaka, Hiroki
Herr, Simon J.
Buse, Karsten
Breunig, Ingo
Optics
Barium magnesium fluoride (BMF) is a ferroelectric crystal with a transparency range far beyond the one of other optical materials. In particular, its low loss in the deep ultraviolet makes this material an unique candidate for frequency conversion in this spectral range. Due to its relatively weak second-order nonlinearity, a resonant configuration such as an optical whispering gallery would be beneficial. We show that femtosecond-laser based material processing enables the reliable fabrication of BMF whispering gallery resonators with quality factors beyond $10^7$. Their resonance frequencies can be shifted linearly by applying electric fields between the $+c$ and $-c$ faces of the crystal. The slope of the shift is $-0.8$~MHz/(V/mm). It seems that the origin of this shift is piezoelectricity, while the electro-optic effect is negligible. Our results pave the way for millimeter-sized frequency converters in the deep ultraviolet. Furthermore, they indicate that a careful determination of fundamental material properties is still necessary.
title Electrically-induced resonance shifts of whispering gallery resonators made of barium magnesium fluoride
topic Optics
url https://arxiv.org/abs/2506.03873