Acoustic Phonon Characteristics of Gallium Oxide Single Crystals Investigated with Brillouin-Mandelstam Light Scattering Spectroscopy

Fuente: arXiv
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Main Authors: Wright, Dylan, Guzman, Erick, Bijoy, Md. Sabbir Hossen, Wilson, Richard B., Mudiyanselage, Dinusha Herath, Fu, Houqiang, Kargar, Fariborz, Balandin, Alexander A.
Format: Preprint
Published: 2025
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author Wright, Dylan
Guzman, Erick
Bijoy, Md. Sabbir Hossen
Wilson, Richard B.
Mudiyanselage, Dinusha Herath
Fu, Houqiang
Kargar, Fariborz
Balandin, Alexander A.
author_facet Wright, Dylan
Guzman, Erick
Bijoy, Md. Sabbir Hossen
Wilson, Richard B.
Mudiyanselage, Dinusha Herath
Fu, Houqiang
Kargar, Fariborz
Balandin, Alexander A.
contents We report an investigation of the bulk and surface acoustic phonons in gallium oxide ultra-wide bandgap single crystals along various crystallographic directions using Brillouin-Mandelstam spectroscopy. Pronounced anisotropy in the acoustic phonon dispersion and velocities was observed across different crystal orientations. The measured average acoustic phonon velocities for the crystallographic directions of interest are 5,250 m/s and 4,990 m/s. The surface acoustic phonons propagate approximately twice as slowly as the bulk acoustic phonons. Our results suggest that the anisotropy of heat conduction in gallium oxide results from the difference in phonon velocities rather than the phonon lifetime. The obtained information for bulk and surface acoustic phonons can be used for developing accurate theoretical models of phonon scattering and optimization of thermal and electrical transport in this technologically important ultra-wide bandgap semiconductor.
format Preprint
id arxiv_https___arxiv_org_abs_2506_05726
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Acoustic Phonon Characteristics of Gallium Oxide Single Crystals Investigated with Brillouin-Mandelstam Light Scattering Spectroscopy
Wright, Dylan
Guzman, Erick
Bijoy, Md. Sabbir Hossen
Wilson, Richard B.
Mudiyanselage, Dinusha Herath
Fu, Houqiang
Kargar, Fariborz
Balandin, Alexander A.
Materials Science
Other Condensed Matter
We report an investigation of the bulk and surface acoustic phonons in gallium oxide ultra-wide bandgap single crystals along various crystallographic directions using Brillouin-Mandelstam spectroscopy. Pronounced anisotropy in the acoustic phonon dispersion and velocities was observed across different crystal orientations. The measured average acoustic phonon velocities for the crystallographic directions of interest are 5,250 m/s and 4,990 m/s. The surface acoustic phonons propagate approximately twice as slowly as the bulk acoustic phonons. Our results suggest that the anisotropy of heat conduction in gallium oxide results from the difference in phonon velocities rather than the phonon lifetime. The obtained information for bulk and surface acoustic phonons can be used for developing accurate theoretical models of phonon scattering and optimization of thermal and electrical transport in this technologically important ultra-wide bandgap semiconductor.
title Acoustic Phonon Characteristics of Gallium Oxide Single Crystals Investigated with Brillouin-Mandelstam Light Scattering Spectroscopy
topic Materials Science
Other Condensed Matter
url https://arxiv.org/abs/2506.05726