Interferometric measurement of nuclear resonant phase shift with a nanoscale Young double waveguide
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| Main Authors: | , , , , , , , , |
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| Format: | Preprint |
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2025
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| _version_ | 1866914489985662976 |
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| author | Lohse, Leon M. Negi, Ankita Osterhoff, Markus Meyer, Paul Yaroslavtsev, Sergey Chumakov, Aleksandr I. Bocklage, Lars Röhlsberger, Ralf Salditt, Tim |
| author_facet | Lohse, Leon M. Negi, Ankita Osterhoff, Markus Meyer, Paul Yaroslavtsev, Sergey Chumakov, Aleksandr I. Bocklage, Lars Röhlsberger, Ralf Salditt, Tim |
| contents | The phase shift of an electromagnetic wave, imprinted by its interaction with atomic scatterers, is a central quantity in optics and photonics. In particular, it encodes information about optical resonances and photon-matter interaction. While being a routine task in the optical regime, interferometric measurements of phase shifts in the x-ray frequency regime are notoriously challenging due to the short wavelengths and associated stability requirements. As a result, the methods demonstrated to date are unsuitable for nanoscopic systems. Here, we demonstrate a nanoscale interferometer, inspired by Young's double-slit experiment, to measure the dispersive phase shift due to the 14.4 keV nuclear resonance of the Mössbauer isotope $^{57}$Fe coupled to an x-ray waveguide. From the single-photon interference patterns, we precisely extract the phase shifts in the vicinity of the nuclear resonance resolved in photon energy by using Bayesian inference. We find that the combined information from phase shift and absorbance reveals microscopic coupling parameters, which are not accessible from the intensity data alone. The demonstrated principle lays a basis for integrated x-ray interferometric sensors. |
| format | Preprint |
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arxiv_https___arxiv_org_abs_2506_05823 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Interferometric measurement of nuclear resonant phase shift with a nanoscale Young double waveguide Lohse, Leon M. Negi, Ankita Osterhoff, Markus Meyer, Paul Yaroslavtsev, Sergey Chumakov, Aleksandr I. Bocklage, Lars Röhlsberger, Ralf Salditt, Tim Optics The phase shift of an electromagnetic wave, imprinted by its interaction with atomic scatterers, is a central quantity in optics and photonics. In particular, it encodes information about optical resonances and photon-matter interaction. While being a routine task in the optical regime, interferometric measurements of phase shifts in the x-ray frequency regime are notoriously challenging due to the short wavelengths and associated stability requirements. As a result, the methods demonstrated to date are unsuitable for nanoscopic systems. Here, we demonstrate a nanoscale interferometer, inspired by Young's double-slit experiment, to measure the dispersive phase shift due to the 14.4 keV nuclear resonance of the Mössbauer isotope $^{57}$Fe coupled to an x-ray waveguide. From the single-photon interference patterns, we precisely extract the phase shifts in the vicinity of the nuclear resonance resolved in photon energy by using Bayesian inference. We find that the combined information from phase shift and absorbance reveals microscopic coupling parameters, which are not accessible from the intensity data alone. The demonstrated principle lays a basis for integrated x-ray interferometric sensors. |
| title | Interferometric measurement of nuclear resonant phase shift with a nanoscale Young double waveguide |
| topic | Optics |
| url | https://arxiv.org/abs/2506.05823 |