Optical Injection and Detection of Long-Lived Interlayer Excitons in van der Waals Heterostructures

Fuente: arXiv
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Main Authors: Tüğen, Alperen, Seiler, Anna M., Christianen, Arthur, Watanabe, Kenji, Taniguchi, Takashi, Kroner, Martin, İmamoğlu, Ataç
Format: Preprint
Published: 2025
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author Tüğen, Alperen
Seiler, Anna M.
Christianen, Arthur
Watanabe, Kenji
Taniguchi, Takashi
Kroner, Martin
İmamoğlu, Ataç
author_facet Tüğen, Alperen
Seiler, Anna M.
Christianen, Arthur
Watanabe, Kenji
Taniguchi, Takashi
Kroner, Martin
İmamoğlu, Ataç
contents Interlayer excitons in semiconducting bilayers separated by insulating hBN layers constitute a promising platform for investigation of strongly correlated bosonic phases. Here, we report an optical method for the generation and characterization of long-lived interlayer excitons. We confirm the presence of tightly bound interlayer excitons by measuring 1s and 2s intralayer excitons in each layer concurrently. Using a pump-probe technique, we find interlayer exciton lifetimes up to 8.8 $μ$s, increasing with the thickness of the hBN. With optical access to long-lived interlayer excitons, our approach provides a new route to explore degenerate Bose--Fermi mixtures of excitons and itinerant electrons with high spatial and temporal resolution.
format Preprint
id arxiv_https___arxiv_org_abs_2506_06098
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Optical Injection and Detection of Long-Lived Interlayer Excitons in van der Waals Heterostructures
Tüğen, Alperen
Seiler, Anna M.
Christianen, Arthur
Watanabe, Kenji
Taniguchi, Takashi
Kroner, Martin
İmamoğlu, Ataç
Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
Interlayer excitons in semiconducting bilayers separated by insulating hBN layers constitute a promising platform for investigation of strongly correlated bosonic phases. Here, we report an optical method for the generation and characterization of long-lived interlayer excitons. We confirm the presence of tightly bound interlayer excitons by measuring 1s and 2s intralayer excitons in each layer concurrently. Using a pump-probe technique, we find interlayer exciton lifetimes up to 8.8 $μ$s, increasing with the thickness of the hBN. With optical access to long-lived interlayer excitons, our approach provides a new route to explore degenerate Bose--Fermi mixtures of excitons and itinerant electrons with high spatial and temporal resolution.
title Optical Injection and Detection of Long-Lived Interlayer Excitons in van der Waals Heterostructures
topic Mesoscale and Nanoscale Physics
Strongly Correlated Electrons
url https://arxiv.org/abs/2506.06098