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Hauptverfasser: Liu, Xiaoqing, Zeng, Kehan, Wang, Yangshuai, Zhao, Teng
Format: Preprint
Veröffentlicht: 2025
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Online-Zugang:https://arxiv.org/abs/2506.07401
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author Liu, Xiaoqing
Zeng, Kehan
Wang, Yangshuai
Zhao, Teng
author_facet Liu, Xiaoqing
Zeng, Kehan
Wang, Yangshuai
Zhao, Teng
contents Universal machine-learned interatomic potentials (U-MLIPs) have demonstrated effectiveness across diverse atomistic systems but often require fine-tuning for task-specific accuracy. We investigate the fine-tuning of two MACE-based foundation models, MACE-MP-0 and its variant MACE-MP-0b, and identify key insights. Fine-tuning on task-specific datasets enhances accuracy and, in some cases, outperforms models trained from scratch. Additionally, fine-tuned models benefit from faster convergence due to the strong initial predictions provided by the foundation model. The success of fine-tuning also depends on careful dataset selection, which can be optimized through filtering or active learning. We further discuss practical strategies for achieving better fine-tuning foundation models in atomistic simulations and explore future directions for their development and applications.
format Preprint
id arxiv_https___arxiv_org_abs_2506_07401
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle A Study on the Fine-Tuning Performance of Universal Machine-Learned Interatomic Potentials (U-MLIPs)
Liu, Xiaoqing
Zeng, Kehan
Wang, Yangshuai
Zhao, Teng
Computational Physics
Universal machine-learned interatomic potentials (U-MLIPs) have demonstrated effectiveness across diverse atomistic systems but often require fine-tuning for task-specific accuracy. We investigate the fine-tuning of two MACE-based foundation models, MACE-MP-0 and its variant MACE-MP-0b, and identify key insights. Fine-tuning on task-specific datasets enhances accuracy and, in some cases, outperforms models trained from scratch. Additionally, fine-tuned models benefit from faster convergence due to the strong initial predictions provided by the foundation model. The success of fine-tuning also depends on careful dataset selection, which can be optimized through filtering or active learning. We further discuss practical strategies for achieving better fine-tuning foundation models in atomistic simulations and explore future directions for their development and applications.
title A Study on the Fine-Tuning Performance of Universal Machine-Learned Interatomic Potentials (U-MLIPs)
topic Computational Physics
url https://arxiv.org/abs/2506.07401