$d$-Wave Flat Fermi Surface in Altermagnets Enables Maximum Charge-to-Spin Conversion

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Hauptverfasser: Lai, Junwen, Yu, Tianye, Liu, Peitao, Liu, Long, Xing, Guozhong, Chen, Xing-Qiu, Sun, Yan
Format: Preprint
Veröffentlicht: 2025
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author Lai, Junwen
Yu, Tianye
Liu, Peitao
Liu, Long
Xing, Guozhong
Chen, Xing-Qiu
Sun, Yan
author_facet Lai, Junwen
Yu, Tianye
Liu, Peitao
Liu, Long
Xing, Guozhong
Chen, Xing-Qiu
Sun, Yan
contents Altermagnets combine antiferromagnetic order with ferromagnet-like spin splitting, a duality that unlocks ultrafast spin-dependent responses. This unique property creates unprecedented opportunities for spin-current generation, overcoming the intrinsic limitations of conventional spin-transfer and spin-orbit torque approaches in magnetic memory technologies. Here, we establish a fundamental relationship between Fermi surface geometry and time-reversal-odd ($\mathcal{T}$-odd) spin currents in altermagnets through combined model analysis and first-principles calculations. We demonstrate that a $d$-wave altermagnet with a flat Fermi surface can achieve a theoretical upper limit of charge-to-spin conversion efficiency (CSE) of 100%. This mechanism is realized in the newly discovered room-temperature altermagnetic metal KV$_2$O$_2$Se, which exhibits a CSE of $\sim$78% at the charge neutrality point, nearly double that of RuO$_2$, setting a new record for $\mathcal{T}$-odd CSE. Under electron doping, this efficiency further increases to $\sim$98%, approaching the theoretical limit. Our work advances the fundamental understanding of $\mathcal{T}$-odd spin currents via Fermi surface geometry engineering and provides key insights for developing next-generation altermagnet-based memory devices.
format Preprint
id arxiv_https___arxiv_org_abs_2506_07703
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle $d$-Wave Flat Fermi Surface in Altermagnets Enables Maximum Charge-to-Spin Conversion
Lai, Junwen
Yu, Tianye
Liu, Peitao
Liu, Long
Xing, Guozhong
Chen, Xing-Qiu
Sun, Yan
Materials Science
Altermagnets combine antiferromagnetic order with ferromagnet-like spin splitting, a duality that unlocks ultrafast spin-dependent responses. This unique property creates unprecedented opportunities for spin-current generation, overcoming the intrinsic limitations of conventional spin-transfer and spin-orbit torque approaches in magnetic memory technologies. Here, we establish a fundamental relationship between Fermi surface geometry and time-reversal-odd ($\mathcal{T}$-odd) spin currents in altermagnets through combined model analysis and first-principles calculations. We demonstrate that a $d$-wave altermagnet with a flat Fermi surface can achieve a theoretical upper limit of charge-to-spin conversion efficiency (CSE) of 100%. This mechanism is realized in the newly discovered room-temperature altermagnetic metal KV$_2$O$_2$Se, which exhibits a CSE of $\sim$78% at the charge neutrality point, nearly double that of RuO$_2$, setting a new record for $\mathcal{T}$-odd CSE. Under electron doping, this efficiency further increases to $\sim$98%, approaching the theoretical limit. Our work advances the fundamental understanding of $\mathcal{T}$-odd spin currents via Fermi surface geometry engineering and provides key insights for developing next-generation altermagnet-based memory devices.
title $d$-Wave Flat Fermi Surface in Altermagnets Enables Maximum Charge-to-Spin Conversion
topic Materials Science
url https://arxiv.org/abs/2506.07703