Erbium-implanted WS2 flakes with room-temperature photon emission at telecom wavelengths

Fuente: arXiv
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Main Authors: García-Arellano, Guadalupe, Morales, Gabriel I. López, Shotan, Zav, Kumar, Raman, Murdin, Ben, Dreyer, Cyrus E., Meriles, Carlos A.
Format: Preprint
Published: 2025
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author García-Arellano, Guadalupe
Morales, Gabriel I. López
Shotan, Zav
Kumar, Raman
Murdin, Ben
Dreyer, Cyrus E.
Meriles, Carlos A.
author_facet García-Arellano, Guadalupe
Morales, Gabriel I. López
Shotan, Zav
Kumar, Raman
Murdin, Ben
Dreyer, Cyrus E.
Meriles, Carlos A.
contents Optically addressable spin impurities in crystals along with device engineering provide an attractive route to realizing quantum technologies in the solid state, but reconciling disparate emitter and host material constraints for a given target application is often challenging. Rare-earth ions in two-dimensional (2D) materials could mitigate this problem given the atomic-like transitions of the emitters and the versatile nature of van der Waals systems. Here we combine ion implantation, confocal microscopy, and ab-initio calculations to examine the photon emission of Er-doped WS2 flakes. Optical spectroscopy reveals narrow, long-lived photo-luminescence lines in the telecom band, which we activate after low-temperature thermal annealing. Spectroscopic and polarization-selective measurements show a uniform response across the ensemble, while the fluorescence brightness remains mostly unchanged with temperature, suggesting non-radiative relaxation channels are inefficient. Our results create opportunities for novel solid state devices coupling 2D-hosted, telecom-band emitters to photonic heterostructures separately optimized for photon manipulation.
format Preprint
id arxiv_https___arxiv_org_abs_2506_07746
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Erbium-implanted WS2 flakes with room-temperature photon emission at telecom wavelengths
García-Arellano, Guadalupe
Morales, Gabriel I. López
Shotan, Zav
Kumar, Raman
Murdin, Ben
Dreyer, Cyrus E.
Meriles, Carlos A.
Mesoscale and Nanoscale Physics
Optically addressable spin impurities in crystals along with device engineering provide an attractive route to realizing quantum technologies in the solid state, but reconciling disparate emitter and host material constraints for a given target application is often challenging. Rare-earth ions in two-dimensional (2D) materials could mitigate this problem given the atomic-like transitions of the emitters and the versatile nature of van der Waals systems. Here we combine ion implantation, confocal microscopy, and ab-initio calculations to examine the photon emission of Er-doped WS2 flakes. Optical spectroscopy reveals narrow, long-lived photo-luminescence lines in the telecom band, which we activate after low-temperature thermal annealing. Spectroscopic and polarization-selective measurements show a uniform response across the ensemble, while the fluorescence brightness remains mostly unchanged with temperature, suggesting non-radiative relaxation channels are inefficient. Our results create opportunities for novel solid state devices coupling 2D-hosted, telecom-band emitters to photonic heterostructures separately optimized for photon manipulation.
title Erbium-implanted WS2 flakes with room-temperature photon emission at telecom wavelengths
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2506.07746