Optical spin pumping in silicon

Fuente: arXiv
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Auteurs principaux: Achilli, Stefano, Marian, Damiano, Lodari, Mario, Bonera, Emiliano, Scappucci, Giordano, Pedrini, Jacopo, Virgilio, Michele, Pezzoli, Fabio
Format: Preprint
Publié: 2025
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author Achilli, Stefano
Marian, Damiano
Lodari, Mario
Bonera, Emiliano
Scappucci, Giordano
Pedrini, Jacopo
Virgilio, Michele
Pezzoli, Fabio
author_facet Achilli, Stefano
Marian, Damiano
Lodari, Mario
Bonera, Emiliano
Scappucci, Giordano
Pedrini, Jacopo
Virgilio, Michele
Pezzoli, Fabio
contents The generation of an out-of-equilibrium population of spin-polarized carriers is a keystone process for quantum technologies and spintronics alike. It can be achieved through the so-called optical spin orientation by exciting the material with circularly polarized light. Although this is an established technique for studying direct band-gap semiconductors, it has been proven limited in materials like Si that possess weak oscillator strengths for the optical transitions. In this study, we address the problem by presenting an all-optical analog of the spin pumping method. This involves the optical creation of a non-equilibrium spin population within an absorber, which subsequently transfers spin-polarized carriers to a nearby indirect gap semiconductor, resulting in polarized emission from the latter. By applying this concept to a Ge-on-Si heterostructure we observe luminescence from Si with an unrivaled polarization degree as high as 9%. The progressive etching of the absorbing layer, assisted by magneto-optic experiments, allows us to ascertain that the polarized emission is determined by effective spin injection aided by the carrier lifetime shortening due to extended defects. These findings can facilitate the use of highly promising spin-dependent phenomena of Si, whose optical exploitation has thus far been hampered by fundamental limitations associated with its peculiar electronic structure.
format Preprint
id arxiv_https___arxiv_org_abs_2506_09926
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Optical spin pumping in silicon
Achilli, Stefano
Marian, Damiano
Lodari, Mario
Bonera, Emiliano
Scappucci, Giordano
Pedrini, Jacopo
Virgilio, Michele
Pezzoli, Fabio
Mesoscale and Nanoscale Physics
Materials Science
The generation of an out-of-equilibrium population of spin-polarized carriers is a keystone process for quantum technologies and spintronics alike. It can be achieved through the so-called optical spin orientation by exciting the material with circularly polarized light. Although this is an established technique for studying direct band-gap semiconductors, it has been proven limited in materials like Si that possess weak oscillator strengths for the optical transitions. In this study, we address the problem by presenting an all-optical analog of the spin pumping method. This involves the optical creation of a non-equilibrium spin population within an absorber, which subsequently transfers spin-polarized carriers to a nearby indirect gap semiconductor, resulting in polarized emission from the latter. By applying this concept to a Ge-on-Si heterostructure we observe luminescence from Si with an unrivaled polarization degree as high as 9%. The progressive etching of the absorbing layer, assisted by magneto-optic experiments, allows us to ascertain that the polarized emission is determined by effective spin injection aided by the carrier lifetime shortening due to extended defects. These findings can facilitate the use of highly promising spin-dependent phenomena of Si, whose optical exploitation has thus far been hampered by fundamental limitations associated with its peculiar electronic structure.
title Optical spin pumping in silicon
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2506.09926