Laser Stabilised Ionising Transitions

Fuente: arXiv
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Autori principali: Cortese, Erika, De Liberato, Simone
Natura: Preprint
Pubblicazione: 2025
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author Cortese, Erika
De Liberato, Simone
author_facet Cortese, Erika
De Liberato, Simone
contents We investigate a ionising electronic transition under resonant pumping. We demonstrate that, above a critical value of the pump intensity, a novel metastable electronic bound state is created, which can decay into the free electron continuum by two-photon ionization. We calculate the system's resonant fluorescence spectrum, finding results qualitatively different from the Mollow triplet expected in a bound-to-bound transition. The fluorescent emission can be used to measure the time-resolved population of the novel metastable state. Contrary to Kramers-Hennenberger atoms, stabilised by non-perturbative, non-resonant laser pulses, the physics we observe is inherently resonant and relies on perturbative level repulsion. In analogy to how the AC-Stark shift is a semiclassical version of the single-photon Rabi splitting observed in photonic cavity, the phenomenon we describe is better understood as a semiclassical version of recently observed excitons bound by a single cavity photon. Our results demonstrate a novel way to stabilise electronic states with intense laser fields, increasing our capability to design and engineer non-classical states of matter.
format Preprint
id arxiv_https___arxiv_org_abs_2506_10183
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Laser Stabilised Ionising Transitions
Cortese, Erika
De Liberato, Simone
Atomic Physics
Other Condensed Matter
Optics
We investigate a ionising electronic transition under resonant pumping. We demonstrate that, above a critical value of the pump intensity, a novel metastable electronic bound state is created, which can decay into the free electron continuum by two-photon ionization. We calculate the system's resonant fluorescence spectrum, finding results qualitatively different from the Mollow triplet expected in a bound-to-bound transition. The fluorescent emission can be used to measure the time-resolved population of the novel metastable state. Contrary to Kramers-Hennenberger atoms, stabilised by non-perturbative, non-resonant laser pulses, the physics we observe is inherently resonant and relies on perturbative level repulsion. In analogy to how the AC-Stark shift is a semiclassical version of the single-photon Rabi splitting observed in photonic cavity, the phenomenon we describe is better understood as a semiclassical version of recently observed excitons bound by a single cavity photon. Our results demonstrate a novel way to stabilise electronic states with intense laser fields, increasing our capability to design and engineer non-classical states of matter.
title Laser Stabilised Ionising Transitions
topic Atomic Physics
Other Condensed Matter
Optics
url https://arxiv.org/abs/2506.10183