From stripes to hexagons: strain-induced 2D Pb phases confined between graphene and SiC

Fuente: arXiv
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Autori principali: Gruschwitz, Markus, Sologub, Sergii, Ghosal, Chitran, Mamiyev, Zamin, Niu, Yuran, Zakharov, Alexei, Tegenkamp, Christoph
Natura: Preprint
Pubblicazione: 2025
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author Gruschwitz, Markus
Sologub, Sergii
Ghosal, Chitran
Mamiyev, Zamin
Niu, Yuran
Zakharov, Alexei
Tegenkamp, Christoph
author_facet Gruschwitz, Markus
Sologub, Sergii
Ghosal, Chitran
Mamiyev, Zamin
Niu, Yuran
Zakharov, Alexei
Tegenkamp, Christoph
contents The intercalation of metals beneath graphene offers a powerful route to stabilizing and protecting novel two-dimensional (2D) phases. The epitaxial growth of Pb monolayers on SiC(0001), combined with the relatively large spacing of the suspended graphene, makes this system particularly distinctive. Using low-energy electron diffraction (LEED) and various microscopy techniques -- including scanning electron microscopy (SEM), scanning tunneling microscopy (STM), and low-energy electron microscopy (LEEM) -- we have investigated the intercalation process across multiple length scales. Our analysis reveals the formation of different 2D Pb monolayer phases, such as stripes and hexagons, which emerge due to the interplay between substrate pinning and strain within the Pb layer, depending on local coverage. These findings provide new insights into the strain-driven stabilization of intercalated metal layers and highlight the potential of graphene as a versatile platform for engineering low-dimensional materials.
format Preprint
id arxiv_https___arxiv_org_abs_2506_10791
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle From stripes to hexagons: strain-induced 2D Pb phases confined between graphene and SiC
Gruschwitz, Markus
Sologub, Sergii
Ghosal, Chitran
Mamiyev, Zamin
Niu, Yuran
Zakharov, Alexei
Tegenkamp, Christoph
Materials Science
Mesoscale and Nanoscale Physics
The intercalation of metals beneath graphene offers a powerful route to stabilizing and protecting novel two-dimensional (2D) phases. The epitaxial growth of Pb monolayers on SiC(0001), combined with the relatively large spacing of the suspended graphene, makes this system particularly distinctive. Using low-energy electron diffraction (LEED) and various microscopy techniques -- including scanning electron microscopy (SEM), scanning tunneling microscopy (STM), and low-energy electron microscopy (LEEM) -- we have investigated the intercalation process across multiple length scales. Our analysis reveals the formation of different 2D Pb monolayer phases, such as stripes and hexagons, which emerge due to the interplay between substrate pinning and strain within the Pb layer, depending on local coverage. These findings provide new insights into the strain-driven stabilization of intercalated metal layers and highlight the potential of graphene as a versatile platform for engineering low-dimensional materials.
title From stripes to hexagons: strain-induced 2D Pb phases confined between graphene and SiC
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2506.10791