Interface-controlled antiferromagnetic tunnel junctions

Fuente: arXiv
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Hauptverfasser: Yang, Liu, Jiang, Yuan-Yuan, Guo, Xiao-Yan, Zhang, Shu-Hui, Xiao, Rui-Chun, Lu, Wen-Jian, Wang, Lan, Sun, Yu-Ping, Tsymbal, Evgeny Y., Shao, Ding-Fu
Format: Preprint
Veröffentlicht: 2025
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author Yang, Liu
Jiang, Yuan-Yuan
Guo, Xiao-Yan
Zhang, Shu-Hui
Xiao, Rui-Chun
Lu, Wen-Jian
Wang, Lan
Sun, Yu-Ping
Tsymbal, Evgeny Y.
Shao, Ding-Fu
author_facet Yang, Liu
Jiang, Yuan-Yuan
Guo, Xiao-Yan
Zhang, Shu-Hui
Xiao, Rui-Chun
Lu, Wen-Jian
Wang, Lan
Sun, Yu-Ping
Tsymbal, Evgeny Y.
Shao, Ding-Fu
contents Magnetic tunnel junctions (MTJs) are the key building blocks of high-performance spintronic devices. While conventional MTJs rely on ferromagnetic (FM) materials, employing antiferromagnetic (AFM) compounds can significantly increase operation speed and packing density. Current prototypes of AFM tunnel junctions (AFMTJs) exploit antiferromagnets either as spin-filter insulating barriers or as metal electrodes supporting bulk spin-dependent currents. Here, we highlight a largely overlooked AFMTJ prototype, where bulk-spin-degenerate electrodes with an A-type AFM stacking form magnetically uncompensated interfaces, enabling spin-polarized tunneling currents and a sizable tunneling magnetoresistance (TMR) effect. Using first-principles quantum-transport calculations and the van der Waals (vdW) metal Fe$_{4}$GeTe$_{2}$ as a representative A-type AFM electrode, we demonstrate a large negative TMR arising solely from the alignment of interfacial magnetic moments. This prototype of AFMTJs can also be realized with various non-vdW A-type AFM metals that support roughness-insensitive surface magnetization. Beyond TMR, AFMTJs based on A-type antiferromagnets allow convenient switching of the Néel vector, opening a new paradigm for AFM spintronics that leverages spin-dependent properties at AFM interfaces.
format Preprint
id arxiv_https___arxiv_org_abs_2506_12715
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Interface-controlled antiferromagnetic tunnel junctions
Yang, Liu
Jiang, Yuan-Yuan
Guo, Xiao-Yan
Zhang, Shu-Hui
Xiao, Rui-Chun
Lu, Wen-Jian
Wang, Lan
Sun, Yu-Ping
Tsymbal, Evgeny Y.
Shao, Ding-Fu
Materials Science
Mesoscale and Nanoscale Physics
Magnetic tunnel junctions (MTJs) are the key building blocks of high-performance spintronic devices. While conventional MTJs rely on ferromagnetic (FM) materials, employing antiferromagnetic (AFM) compounds can significantly increase operation speed and packing density. Current prototypes of AFM tunnel junctions (AFMTJs) exploit antiferromagnets either as spin-filter insulating barriers or as metal electrodes supporting bulk spin-dependent currents. Here, we highlight a largely overlooked AFMTJ prototype, where bulk-spin-degenerate electrodes with an A-type AFM stacking form magnetically uncompensated interfaces, enabling spin-polarized tunneling currents and a sizable tunneling magnetoresistance (TMR) effect. Using first-principles quantum-transport calculations and the van der Waals (vdW) metal Fe$_{4}$GeTe$_{2}$ as a representative A-type AFM electrode, we demonstrate a large negative TMR arising solely from the alignment of interfacial magnetic moments. This prototype of AFMTJs can also be realized with various non-vdW A-type AFM metals that support roughness-insensitive surface magnetization. Beyond TMR, AFMTJs based on A-type antiferromagnets allow convenient switching of the Néel vector, opening a new paradigm for AFM spintronics that leverages spin-dependent properties at AFM interfaces.
title Interface-controlled antiferromagnetic tunnel junctions
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2506.12715