Disorder-Engineered Hybrid Plasmonic Cavities for Emission Control of Defects in hBN
Fuente:
arXiv
Saved in:
| Main Authors: | , , , , , , , |
|---|---|
| Format: | Preprint |
| Published: |
2025
|
| Subjects: | |
| Online Access: | |
| Tags: |
Add Tag
No Tags, Be the first to tag this record!
|
| _version_ | 1866918437128765440 |
|---|---|
| author | Genc, Sinan Yucel, Oguzhan Aglarci, Furkan Rodriguez-Fernandez, Carlos Yilmaz, Alpay Caglayan, Humeyra Ates, Serkan Bek, Alpan |
| author_facet | Genc, Sinan Yucel, Oguzhan Aglarci, Furkan Rodriguez-Fernandez, Carlos Yilmaz, Alpay Caglayan, Humeyra Ates, Serkan Bek, Alpan |
| contents | Defect-based quantum emitters in hexagonal boron nitride (hBN) are promising building blocks for scalable quantum photonics due to their stable single-photon emission at room temperature. However, enhancing their emission intensity and controlling the decay dynamics remain significant challenges. This study demonstrates a low-cost, scalable fabrication approach to integrate plasmonic nanocavities with defect-based quantum emitters in hBN nanoflakes. Using the thermal dewetting process, we realize two distinct configurations: stochastic Ag nanoparticles (AgNPs) on hBN flakes and hybrid plasmonic nanocavities formed by AgNPs on top of hBN flakes supported on gold/silicon dioxide (Au/SiO2) substrates. While AgNPs on bare hBN yield up to a two-fold photoluminescence (PL) enhancement with reduced emitter lifetimes, the hybrid nanocavity architecture provides a dramatic, up to 100-fold PL enhancement and improved uniformity across multiple. emitters, all without requiring deterministic positioning. Finite-difference time-domain (FDTD) simulations and time-resolved PL measurements confirm size-dependent control over decay dynamics and cavity-emitter interactions. Our versatile solution overcomes key quantum photonic device development challenges, including material integration, emission intensity optimization, and spectral multiplexity. Future work will explore potential applications in integrated photonic circuits hosting on-chip quantum systems and hBN-based label-free single-molecule detection through such quantum nanoantennas. |
| format | Preprint |
| id |
arxiv_https___arxiv_org_abs_2506_14517 |
| institution | arXiv |
| publishDate | 2025 |
| record_format | arxiv |
| spellingShingle | Disorder-Engineered Hybrid Plasmonic Cavities for Emission Control of Defects in hBN Genc, Sinan Yucel, Oguzhan Aglarci, Furkan Rodriguez-Fernandez, Carlos Yilmaz, Alpay Caglayan, Humeyra Ates, Serkan Bek, Alpan Optics Applied Physics Quantum Physics Defect-based quantum emitters in hexagonal boron nitride (hBN) are promising building blocks for scalable quantum photonics due to their stable single-photon emission at room temperature. However, enhancing their emission intensity and controlling the decay dynamics remain significant challenges. This study demonstrates a low-cost, scalable fabrication approach to integrate plasmonic nanocavities with defect-based quantum emitters in hBN nanoflakes. Using the thermal dewetting process, we realize two distinct configurations: stochastic Ag nanoparticles (AgNPs) on hBN flakes and hybrid plasmonic nanocavities formed by AgNPs on top of hBN flakes supported on gold/silicon dioxide (Au/SiO2) substrates. While AgNPs on bare hBN yield up to a two-fold photoluminescence (PL) enhancement with reduced emitter lifetimes, the hybrid nanocavity architecture provides a dramatic, up to 100-fold PL enhancement and improved uniformity across multiple. emitters, all without requiring deterministic positioning. Finite-difference time-domain (FDTD) simulations and time-resolved PL measurements confirm size-dependent control over decay dynamics and cavity-emitter interactions. Our versatile solution overcomes key quantum photonic device development challenges, including material integration, emission intensity optimization, and spectral multiplexity. Future work will explore potential applications in integrated photonic circuits hosting on-chip quantum systems and hBN-based label-free single-molecule detection through such quantum nanoantennas. |
| title | Disorder-Engineered Hybrid Plasmonic Cavities for Emission Control of Defects in hBN |
| topic | Optics Applied Physics Quantum Physics |
| url | https://arxiv.org/abs/2506.14517 |