Ultrafast dynamics of three-dimensional Kane plasmons in the narrow-bandgap Hg$_{0.8}$Cd$_{0.2}$Te

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Main Authors: Zhou, Xiaoyue, Chan, Yi, Zhu, Siyuan, Deng, Fu, Bai, Wei, Zhang, Jingdi
Format: Preprint
Published: 2025
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author Zhou, Xiaoyue
Chan, Yi
Zhu, Siyuan
Deng, Fu
Bai, Wei
Zhang, Jingdi
author_facet Zhou, Xiaoyue
Chan, Yi
Zhu, Siyuan
Deng, Fu
Bai, Wei
Zhang, Jingdi
contents We report on an ultrafast terahertz spectroscopic study on the dynamics of free carriers and the pertinent bulk plasmons in Hg$_{0.8}$Cd$_{0.2}$Te (MCT) film, a narrowband semiconductor accommodating three dimensional massless Kane fermions. The ultrabroadband terahertz source enables the investigation of the lightly doped equilibrium state in the presence of plasmon-phonon hybridization through the heavily doped excited state, primarily dominated by plasmons. Without the recourse to the resource consuming cryogenic high magnetic field spectroscopy that hinges on observable related to the interband transition, we show that the massless band dispersion can instead be conveniently perceived by the room temperature study of the intraband transition through the determination of the plasmon carrier density relationship. We found the plasma frequency in MCT scales with the cube root of carrier density, in contrast with the square root scaling in the conventional massive fermion system of parabolic band dispersion. This work also answers the curious question of whether the MCT can maintain its massless Kane fermion character in case the strict gapless condition is deviated from. The method presented herein provides a convenient approach to identifying the landscape of both massless and massive band dispersion.
format Preprint
id arxiv_https___arxiv_org_abs_2506_16049
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Ultrafast dynamics of three-dimensional Kane plasmons in the narrow-bandgap Hg$_{0.8}$Cd$_{0.2}$Te
Zhou, Xiaoyue
Chan, Yi
Zhu, Siyuan
Deng, Fu
Bai, Wei
Zhang, Jingdi
Materials Science
Mesoscale and Nanoscale Physics
We report on an ultrafast terahertz spectroscopic study on the dynamics of free carriers and the pertinent bulk plasmons in Hg$_{0.8}$Cd$_{0.2}$Te (MCT) film, a narrowband semiconductor accommodating three dimensional massless Kane fermions. The ultrabroadband terahertz source enables the investigation of the lightly doped equilibrium state in the presence of plasmon-phonon hybridization through the heavily doped excited state, primarily dominated by plasmons. Without the recourse to the resource consuming cryogenic high magnetic field spectroscopy that hinges on observable related to the interband transition, we show that the massless band dispersion can instead be conveniently perceived by the room temperature study of the intraband transition through the determination of the plasmon carrier density relationship. We found the plasma frequency in MCT scales with the cube root of carrier density, in contrast with the square root scaling in the conventional massive fermion system of parabolic band dispersion. This work also answers the curious question of whether the MCT can maintain its massless Kane fermion character in case the strict gapless condition is deviated from. The method presented herein provides a convenient approach to identifying the landscape of both massless and massive band dispersion.
title Ultrafast dynamics of three-dimensional Kane plasmons in the narrow-bandgap Hg$_{0.8}$Cd$_{0.2}$Te
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2506.16049