Superconducting critical temperature and dimensionality tuning of RbV$_3$Sb$_5$ via biaxial strain

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Main Authors: Poon, Tsz Fung, Yip, King Yau, Tsui, Ying Kit, Wang, Lingfei, Yu, Kai Ham, Zhang, Wei, Wang, Zheyu, Nakatani, Taketo, Michioka, Chishiro, Ueda, Hiroaki, Lam, Siu Tung, Lai, Kwing To, Goh, Swee K.
Format: Preprint
Published: 2025
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author Poon, Tsz Fung
Yip, King Yau
Tsui, Ying Kit
Wang, Lingfei
Yu, Kai Ham
Zhang, Wei
Wang, Zheyu
Nakatani, Taketo
Michioka, Chishiro
Ueda, Hiroaki
Lam, Siu Tung
Lai, Kwing To
Goh, Swee K.
author_facet Poon, Tsz Fung
Yip, King Yau
Tsui, Ying Kit
Wang, Lingfei
Yu, Kai Ham
Zhang, Wei
Wang, Zheyu
Nakatani, Taketo
Michioka, Chishiro
Ueda, Hiroaki
Lam, Siu Tung
Lai, Kwing To
Goh, Swee K.
contents Kagome metal AV$_3$Sb$_5$ (A=K, Rb, Cs) has emerged as an intriguing platform for exploring the interplay between superconductivity and other quantum states. Among the three compounds, RbV$_3$Sb$_5$ has a notably lower superconducting critical temperature ($T_c$) at ambient pressure, posing challenges in exploring the superconducting state. For instance, the upper critical field ($H_{c2}$) is small and thus difficult to measure accurately against other control parameters. Hence, enhancing superconductivity would facilitate $H_{c2}$ measurements, providing insights into key superconducting properties such as the dimensionality. In this letter, we report the tuning of the $T_c$ in RbV$_3$Sb$_5$ through the application of biaxial strain. Utilizing a negative thermal expansion material ZrW$_2$O$_8$ as a substrate, we achieve a substantial biaxial strain of $ε=1.50\%$, resulting in a remarkable 75\% enhancement in $T_c$. We investigate the $H_{c2}$ as a function of temperature, revealing a transition from multi-band to single-band superconductivity with increasing tensile strain. Additionally, we study the $H_{c2}$ as a function of field angle, revealing a plausible correlation between the $T_c$ enhancement and the change in dimensionality of the superconductivity under tensile strain. Further analysis quantitatively illustrates a transition towards two-dimensional superconductivity in RbV$_3$Sb$_5$ when subjected to tensile strain. Our work demonstrates that the application of biaxial strain allows for the tuning of both the $T_c$ and superconducting dimensionality in RbV$_3$Sb$_5$.
format Preprint
id arxiv_https___arxiv_org_abs_2506_16165
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Superconducting critical temperature and dimensionality tuning of RbV$_3$Sb$_5$ via biaxial strain
Poon, Tsz Fung
Yip, King Yau
Tsui, Ying Kit
Wang, Lingfei
Yu, Kai Ham
Zhang, Wei
Wang, Zheyu
Nakatani, Taketo
Michioka, Chishiro
Ueda, Hiroaki
Lam, Siu Tung
Lai, Kwing To
Goh, Swee K.
Superconductivity
Materials Science
Kagome metal AV$_3$Sb$_5$ (A=K, Rb, Cs) has emerged as an intriguing platform for exploring the interplay between superconductivity and other quantum states. Among the three compounds, RbV$_3$Sb$_5$ has a notably lower superconducting critical temperature ($T_c$) at ambient pressure, posing challenges in exploring the superconducting state. For instance, the upper critical field ($H_{c2}$) is small and thus difficult to measure accurately against other control parameters. Hence, enhancing superconductivity would facilitate $H_{c2}$ measurements, providing insights into key superconducting properties such as the dimensionality. In this letter, we report the tuning of the $T_c$ in RbV$_3$Sb$_5$ through the application of biaxial strain. Utilizing a negative thermal expansion material ZrW$_2$O$_8$ as a substrate, we achieve a substantial biaxial strain of $ε=1.50\%$, resulting in a remarkable 75\% enhancement in $T_c$. We investigate the $H_{c2}$ as a function of temperature, revealing a transition from multi-band to single-band superconductivity with increasing tensile strain. Additionally, we study the $H_{c2}$ as a function of field angle, revealing a plausible correlation between the $T_c$ enhancement and the change in dimensionality of the superconductivity under tensile strain. Further analysis quantitatively illustrates a transition towards two-dimensional superconductivity in RbV$_3$Sb$_5$ when subjected to tensile strain. Our work demonstrates that the application of biaxial strain allows for the tuning of both the $T_c$ and superconducting dimensionality in RbV$_3$Sb$_5$.
title Superconducting critical temperature and dimensionality tuning of RbV$_3$Sb$_5$ via biaxial strain
topic Superconductivity
Materials Science
url https://arxiv.org/abs/2506.16165