Laser-induced ultrafast structural transformations in thin Fe layer revealed by time-resolved X-ray diffraction

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Hauptverfasser: Liubchenko, O., Antonowicz, J., Sokolowski-Tinten, K., Zalden, P., Minikayev, R., Milov, I., Albert, T. J., Bressler, C., Chojnacki, M., Dłużewski, P., Dzięgielewski, P., Rodriguez-Fernandez, A., Fronc, K., Gawelda, W., Georgarakis, K., Greer, A. L., Jacyna, I., van de Kruijs, R. W. E., Kamiński, R., Khakhulin, D., Klinger, D., Kosyl, K., Kubicek, K., Olczak, A., Panagiotopoulos, N. T., Sikora, M., Sun, P., Yousef, H., Zajkowska-Pietrzak, W., Sobierajski, R.
Format: Preprint
Veröffentlicht: 2025
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author Liubchenko, O.
Antonowicz, J.
Sokolowski-Tinten, K.
Zalden, P.
Minikayev, R.
Milov, I.
Albert, T. J.
Bressler, C.
Chojnacki, M.
Dłużewski, P.
Dzięgielewski, P.
Rodriguez-Fernandez, A.
Fronc, K.
Gawelda, W.
Georgarakis, K.
Greer, A. L.
Jacyna, I.
van de Kruijs, R. W. E.
Kamiński, R.
Khakhulin, D.
Klinger, D.
Kosyl, K.
Kubicek, K.
Olczak, A.
Panagiotopoulos, N. T.
Sikora, M.
Sun, P.
Yousef, H.
Zajkowska-Pietrzak, W.
Sobierajski, R.
author_facet Liubchenko, O.
Antonowicz, J.
Sokolowski-Tinten, K.
Zalden, P.
Minikayev, R.
Milov, I.
Albert, T. J.
Bressler, C.
Chojnacki, M.
Dłużewski, P.
Dzięgielewski, P.
Rodriguez-Fernandez, A.
Fronc, K.
Gawelda, W.
Georgarakis, K.
Greer, A. L.
Jacyna, I.
van de Kruijs, R. W. E.
Kamiński, R.
Khakhulin, D.
Klinger, D.
Kosyl, K.
Kubicek, K.
Olczak, A.
Panagiotopoulos, N. T.
Sikora, M.
Sun, P.
Yousef, H.
Zajkowska-Pietrzak, W.
Sobierajski, R.
contents The ultrafast structural response of a thin iron film to sub-ps pulsed laser-induced heating has been investigated using time-resolved X-ray diffraction in the partial melting regime. A tetragonal distortion of the bcc-phase emerges at ~6 ps. Its formation is delayed relative to the initial heating (1-2 ps) and partial melting (2-5 ps) of the material, and controlled by the stress release in the quasi-instantaneously pressurized film. The distortion persists for at least 60 ps indicating the formation of a metastable bct phase between the equilibrium bcc and fcc phases.
format Preprint
id arxiv_https___arxiv_org_abs_2506_18730
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Laser-induced ultrafast structural transformations in thin Fe layer revealed by time-resolved X-ray diffraction
Liubchenko, O.
Antonowicz, J.
Sokolowski-Tinten, K.
Zalden, P.
Minikayev, R.
Milov, I.
Albert, T. J.
Bressler, C.
Chojnacki, M.
Dłużewski, P.
Dzięgielewski, P.
Rodriguez-Fernandez, A.
Fronc, K.
Gawelda, W.
Georgarakis, K.
Greer, A. L.
Jacyna, I.
van de Kruijs, R. W. E.
Kamiński, R.
Khakhulin, D.
Klinger, D.
Kosyl, K.
Kubicek, K.
Olczak, A.
Panagiotopoulos, N. T.
Sikora, M.
Sun, P.
Yousef, H.
Zajkowska-Pietrzak, W.
Sobierajski, R.
Materials Science
Mesoscale and Nanoscale Physics
The ultrafast structural response of a thin iron film to sub-ps pulsed laser-induced heating has been investigated using time-resolved X-ray diffraction in the partial melting regime. A tetragonal distortion of the bcc-phase emerges at ~6 ps. Its formation is delayed relative to the initial heating (1-2 ps) and partial melting (2-5 ps) of the material, and controlled by the stress release in the quasi-instantaneously pressurized film. The distortion persists for at least 60 ps indicating the formation of a metastable bct phase between the equilibrium bcc and fcc phases.
title Laser-induced ultrafast structural transformations in thin Fe layer revealed by time-resolved X-ray diffraction
topic Materials Science
Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2506.18730