Real-Space Approach to Light-Induced Hall Transport in Disordered Materials

Fuente: arXiv
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Main Authors: Romeral, Jorge Martinez, Canonico, Luis M., Cummings, Aron W., Roche, Stephan
Format: Preprint
Published: 2025
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author Romeral, Jorge Martinez
Canonico, Luis M.
Cummings, Aron W.
Roche, Stephan
author_facet Romeral, Jorge Martinez
Canonico, Luis M.
Cummings, Aron W.
Roche, Stephan
contents We introduce a linear-scaling real-space methodology to compute time-resolved electrical responses of materials driven far from equilibrium, with energy relaxation and disorder treated on equal footing. Applying this approach to gapped monolayer and AB-stacked (Bernal) bilayer graphene, when driven by a circularly polarized optical pulse, we observe the generation/suppression of a finite Hall conductivity when the system is trivial/topological. This Hall signal oscillates during optical driving and remains sizable after the light is switched off before relaxing toward equilibrium. Remarkably, this dynamical Hall response is robust in the presence of realistic descriptions of disorder, suggesting that disorder and relaxation dynamics can be leveraged as design parameters rather than as limitations. More broadly, our new methodology enables the investigation of electrical responses in driven, complex disordered quantum materials and highlights how engineered energy-transfer pathways can enable ultrafast optoelectronic functionality.
format Preprint
id arxiv_https___arxiv_org_abs_2506_19184
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Real-Space Approach to Light-Induced Hall Transport in Disordered Materials
Romeral, Jorge Martinez
Canonico, Luis M.
Cummings, Aron W.
Roche, Stephan
Mesoscale and Nanoscale Physics
Materials Science
We introduce a linear-scaling real-space methodology to compute time-resolved electrical responses of materials driven far from equilibrium, with energy relaxation and disorder treated on equal footing. Applying this approach to gapped monolayer and AB-stacked (Bernal) bilayer graphene, when driven by a circularly polarized optical pulse, we observe the generation/suppression of a finite Hall conductivity when the system is trivial/topological. This Hall signal oscillates during optical driving and remains sizable after the light is switched off before relaxing toward equilibrium. Remarkably, this dynamical Hall response is robust in the presence of realistic descriptions of disorder, suggesting that disorder and relaxation dynamics can be leveraged as design parameters rather than as limitations. More broadly, our new methodology enables the investigation of electrical responses in driven, complex disordered quantum materials and highlights how engineered energy-transfer pathways can enable ultrafast optoelectronic functionality.
title Real-Space Approach to Light-Induced Hall Transport in Disordered Materials
topic Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2506.19184