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Main Authors: Volpato, Maria Carolina, Estevam, Kalebe B., Davanco, Marcelo I., de Assis, Pierre-Louis
Format: Preprint
Published: 2025
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Online Access:https://arxiv.org/abs/2506.19214
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_version_ 1866915357433790464
author Volpato, Maria Carolina
Estevam, Kalebe B.
Davanco, Marcelo I.
de Assis, Pierre-Louis
author_facet Volpato, Maria Carolina
Estevam, Kalebe B.
Davanco, Marcelo I.
de Assis, Pierre-Louis
contents Horizontal slot waveguides are planar photonic structures with a guided mode which is strongly polarized in the out-of-plane direction and tightly confined in a sub-wavelength region of lower refractive index. We show through FDTD simulations that this mode can lead to coupling efficiencies $β>80\%$ and Purcell factors $F_P>10$ for some types of dark intralayer excitons in transition metal dichalcogenide (TMD) monolayers -- more aplty named ``gray excitons'', as their out-of-plane dipole does couple to adequately polarized light -- as well as interlayer excitons in TMD heterostructures. These figures indicate a path to the strong coupling regime for gray and interlayer excitons, while bright excitons are poorly coupled to the slot mode and experience Purcell suppression for $λ>\SI{1}{\micro\meter}$. A significant hurdle towards strong coupling, however, is the low oscillator strengths of these two excitonic species. We use the Tavis-Cummings model to show that a horizontal-slot racetrack resonator can overcome this difficulty and reach a cooperativity $C>>1$, albeit sacrificing the broadband characteristic of waveguides.
format Preprint
id arxiv_https___arxiv_org_abs_2506_19214
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Broadband photonic structures to achieve high coupling efficiencies and Purcell factors with dark and interlayer excitons in 2D materials
Volpato, Maria Carolina
Estevam, Kalebe B.
Davanco, Marcelo I.
de Assis, Pierre-Louis
Quantum Physics
Horizontal slot waveguides are planar photonic structures with a guided mode which is strongly polarized in the out-of-plane direction and tightly confined in a sub-wavelength region of lower refractive index. We show through FDTD simulations that this mode can lead to coupling efficiencies $β>80\%$ and Purcell factors $F_P>10$ for some types of dark intralayer excitons in transition metal dichalcogenide (TMD) monolayers -- more aplty named ``gray excitons'', as their out-of-plane dipole does couple to adequately polarized light -- as well as interlayer excitons in TMD heterostructures. These figures indicate a path to the strong coupling regime for gray and interlayer excitons, while bright excitons are poorly coupled to the slot mode and experience Purcell suppression for $λ>\SI{1}{\micro\meter}$. A significant hurdle towards strong coupling, however, is the low oscillator strengths of these two excitonic species. We use the Tavis-Cummings model to show that a horizontal-slot racetrack resonator can overcome this difficulty and reach a cooperativity $C>>1$, albeit sacrificing the broadband characteristic of waveguides.
title Broadband photonic structures to achieve high coupling efficiencies and Purcell factors with dark and interlayer excitons in 2D materials
topic Quantum Physics
url https://arxiv.org/abs/2506.19214