Dynamics of Cu$_2$O Rydberg excitons -- real density matrix approach

Fuente: arXiv
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Autores principales: Karpinski, Karol, Czajkowski, Gerard
Formato: Preprint
Publicado: 2025
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author Karpinski, Karol
Czajkowski, Gerard
author_facet Karpinski, Karol
Czajkowski, Gerard
contents Basing on recent reliable measurements of the life- and coherence time of Cu$_2$O Rydberg excitons, we present an analytical method which enables to describe the experimental results. The real-density matrix approach (RDMA) is applied to describe two-photon absorption in Cu$_2$O through the excitonic response to the exciting fields. This approach produces an analytical expression for the emission intensity time evolution, and can be used to explain trends in reported experimental data. Our approach takes into account the effect of the coherence between the electron-hole pair and the electromagnetic fields, the quantum beats and the life- and coherence time dependence on the applied laser power. Adding a separation of slow- and rapid dynamics components we find excellent agreement with the experimental data.
format Preprint
id arxiv_https___arxiv_org_abs_2506_19336
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Dynamics of Cu$_2$O Rydberg excitons -- real density matrix approach
Karpinski, Karol
Czajkowski, Gerard
Mesoscale and Nanoscale Physics
Basing on recent reliable measurements of the life- and coherence time of Cu$_2$O Rydberg excitons, we present an analytical method which enables to describe the experimental results. The real-density matrix approach (RDMA) is applied to describe two-photon absorption in Cu$_2$O through the excitonic response to the exciting fields. This approach produces an analytical expression for the emission intensity time evolution, and can be used to explain trends in reported experimental data. Our approach takes into account the effect of the coherence between the electron-hole pair and the electromagnetic fields, the quantum beats and the life- and coherence time dependence on the applied laser power. Adding a separation of slow- and rapid dynamics components we find excellent agreement with the experimental data.
title Dynamics of Cu$_2$O Rydberg excitons -- real density matrix approach
topic Mesoscale and Nanoscale Physics
url https://arxiv.org/abs/2506.19336