Sparse Infrared Spectroscopy for Detection of Volatile Organic Compounds

Fuente: arXiv
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Main Authors: Welner, Mira, Hazbun, Andre, Beechem, Thomas
Format: Preprint
Published: 2025
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author Welner, Mira
Hazbun, Andre
Beechem, Thomas
author_facet Welner, Mira
Hazbun, Andre
Beechem, Thomas
contents To reduce the complexity of infrared spectroscopy hardware while maintaining performance, a data informed, task-specific, spectral collection approach termed Sparse Infrared Spectroscopy (SIRS) is developed. Using a numerically based virtual experiment based on a quantitatively accurate infrared database, non-negative matrix factorization is used to identify the spectral pass bands of a minimal number of filters necessary to identify volatile organic compounds (VOC) within either an inert background or mixture of gases. The data-driven approach is found capable of identifying contaminants at the 1-10 part per million level (PPM) with $\mathrm{\sim~20-50}$ spectral samples as opposed to the more than 1,000 typical of a traditional infrared spectrum. Reasonably robust to both noise and the characteristics of the base compound in a mixture, the task-specific spectral sampling points to simplified hardware design that maintains performance.
format Preprint
id arxiv_https___arxiv_org_abs_2506_20678
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Sparse Infrared Spectroscopy for Detection of Volatile Organic Compounds
Welner, Mira
Hazbun, Andre
Beechem, Thomas
Chemical Physics
Data Analysis, Statistics and Probability
To reduce the complexity of infrared spectroscopy hardware while maintaining performance, a data informed, task-specific, spectral collection approach termed Sparse Infrared Spectroscopy (SIRS) is developed. Using a numerically based virtual experiment based on a quantitatively accurate infrared database, non-negative matrix factorization is used to identify the spectral pass bands of a minimal number of filters necessary to identify volatile organic compounds (VOC) within either an inert background or mixture of gases. The data-driven approach is found capable of identifying contaminants at the 1-10 part per million level (PPM) with $\mathrm{\sim~20-50}$ spectral samples as opposed to the more than 1,000 typical of a traditional infrared spectrum. Reasonably robust to both noise and the characteristics of the base compound in a mixture, the task-specific spectral sampling points to simplified hardware design that maintains performance.
title Sparse Infrared Spectroscopy for Detection of Volatile Organic Compounds
topic Chemical Physics
Data Analysis, Statistics and Probability
url https://arxiv.org/abs/2506.20678