Imaginary Time Formalism for Causal Nonlinear Response Functions

Fuente: arXiv
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Main Authors: Sinha, Sounak, Bradlyn, Barry
Format: Preprint
Published: 2025
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author Sinha, Sounak
Bradlyn, Barry
author_facet Sinha, Sounak
Bradlyn, Barry
contents It is well established that causal linear response functions can be found by computing the much simpler imaginary time-ordered Matsubara functions and performing an analytic continuation. This principle is the basis for much of our understanding of linear response for interacting and disordered systems, via diagrammatic perturbation theory. Similar imaginary-time approaches have recently been introduced for computing nonlinear response functions as well, although the rigorous connection between Matsubara and causal nonlinear response functions has not been clearly elucidated. In this work, we provide a proof of this connection to all orders in perturbation theory. Using an equations of motion approach, we show by induction that casual nonlinear response functions at every order can be obtained from an analytic continuation of an appropriate time-ordered Matsubara function. We demonstrate this connection explicitly for second order response functions in the Lehmann representation. As a byproduct of our approach, we derive an explicit expression for the Lehmann representation of $n$-th order response functions by solving the equations of motion. We also use our result to find an analytic spectral density representation for both causal response functions and Matsubara functions. Finally, we show how our results lead to a family of generalized sum rules, focusing explicitly on the asymptotic expression for $n$-th harmonic generation rate.
format Preprint
id arxiv_https___arxiv_org_abs_2506_21428
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Imaginary Time Formalism for Causal Nonlinear Response Functions
Sinha, Sounak
Bradlyn, Barry
Mesoscale and Nanoscale Physics
Statistical Mechanics
Quantum Physics
It is well established that causal linear response functions can be found by computing the much simpler imaginary time-ordered Matsubara functions and performing an analytic continuation. This principle is the basis for much of our understanding of linear response for interacting and disordered systems, via diagrammatic perturbation theory. Similar imaginary-time approaches have recently been introduced for computing nonlinear response functions as well, although the rigorous connection between Matsubara and causal nonlinear response functions has not been clearly elucidated. In this work, we provide a proof of this connection to all orders in perturbation theory. Using an equations of motion approach, we show by induction that casual nonlinear response functions at every order can be obtained from an analytic continuation of an appropriate time-ordered Matsubara function. We demonstrate this connection explicitly for second order response functions in the Lehmann representation. As a byproduct of our approach, we derive an explicit expression for the Lehmann representation of $n$-th order response functions by solving the equations of motion. We also use our result to find an analytic spectral density representation for both causal response functions and Matsubara functions. Finally, we show how our results lead to a family of generalized sum rules, focusing explicitly on the asymptotic expression for $n$-th harmonic generation rate.
title Imaginary Time Formalism for Causal Nonlinear Response Functions
topic Mesoscale and Nanoscale Physics
Statistical Mechanics
Quantum Physics
url https://arxiv.org/abs/2506.21428