Optical cycling of MgF molecules within the hyperfine states in X(N=1) state

Fuente: arXiv
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Main Authors: Kwon, Kikyeong, Roh, Seunghwan, Cho, Youngju, Lee, Yongwoong, Chae, Eunmi
Format: Preprint
Published: 2025
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author Kwon, Kikyeong
Roh, Seunghwan
Cho, Youngju
Lee, Yongwoong
Chae, Eunmi
author_facet Kwon, Kikyeong
Roh, Seunghwan
Cho, Youngju
Lee, Yongwoong
Chae, Eunmi
contents We investigated the optical cycling effect of the $\mathrm{X}^2Σ(v=0,\ N=1^-) - \mathrm{A}^2Π_{1/2}(v'=0,\ J'=1/2^+)$ band of MgF molecules, specifically the $\mathrm{P_1/Q_{12}(1)}$ transition, which serves as the main transition in the quasi-closed cycling scheme for the laser cooling. A higher number of scattered photons was observed when all three frequency components of the $\mathrm{P_1/Q_{12}(1)}$ transition were simultaneously applied using acousto-optic modulators (AOMs). Optimal conditions were identified by scanning the detuning of frequency components, the laser beam power ratio, and the total laser beam power, and the results were confirmed through rate equation simulations. Under these optimized conditions, and with an applied magnetic field, the scattering rate was enhanced by approximately a factor of six. These results refine the implementation of optical cycling in MgF and lay the groundwork for laser slowing and magneto-optical trapping (MOT) experiments.
format Preprint
id arxiv_https___arxiv_org_abs_2506_23507
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Optical cycling of MgF molecules within the hyperfine states in X(N=1) state
Kwon, Kikyeong
Roh, Seunghwan
Cho, Youngju
Lee, Yongwoong
Chae, Eunmi
Atomic and Molecular Clusters
Atomic Physics
We investigated the optical cycling effect of the $\mathrm{X}^2Σ(v=0,\ N=1^-) - \mathrm{A}^2Π_{1/2}(v'=0,\ J'=1/2^+)$ band of MgF molecules, specifically the $\mathrm{P_1/Q_{12}(1)}$ transition, which serves as the main transition in the quasi-closed cycling scheme for the laser cooling. A higher number of scattered photons was observed when all three frequency components of the $\mathrm{P_1/Q_{12}(1)}$ transition were simultaneously applied using acousto-optic modulators (AOMs). Optimal conditions were identified by scanning the detuning of frequency components, the laser beam power ratio, and the total laser beam power, and the results were confirmed through rate equation simulations. Under these optimized conditions, and with an applied magnetic field, the scattering rate was enhanced by approximately a factor of six. These results refine the implementation of optical cycling in MgF and lay the groundwork for laser slowing and magneto-optical trapping (MOT) experiments.
title Optical cycling of MgF molecules within the hyperfine states in X(N=1) state
topic Atomic and Molecular Clusters
Atomic Physics
url https://arxiv.org/abs/2506.23507