Enhancement of quantum coherence in solid-state qubits via interface engineering

Fuente: arXiv
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Autores principales: Lo, Wing Ki, Zhang, Yaowen, Chow, Ho Yin, Wu, Jiahao, Leung, Man Yin, Ho, Kin On, Du, Xuliang, Chen, Yifan, Shen, Yang, Pan, Ding, Yang, Sen
Formato: Preprint
Publicado: 2025
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author Lo, Wing Ki
Zhang, Yaowen
Chow, Ho Yin
Wu, Jiahao
Leung, Man Yin
Ho, Kin On
Du, Xuliang
Chen, Yifan
Shen, Yang
Pan, Ding
Yang, Sen
author_facet Lo, Wing Ki
Zhang, Yaowen
Chow, Ho Yin
Wu, Jiahao
Leung, Man Yin
Ho, Kin On
Du, Xuliang
Chen, Yifan
Shen, Yang
Pan, Ding
Yang, Sen
contents Shallow nitrogen-vacancy (NV) centers in diamond are promising quantum sensors but suffer from noise-induced short coherence times due to bulk and surface impurities. We present interfacial engineering via oxygen termination and graphene patching, extending shallow NV coherence to over 1 ms, approaching the T1 limit. Raman spectroscopy and density-functional theory reveal surface termination-driven graphene charge transfer reduces spin noise by pairing surface electrons, supported by double electron-electron resonance spectroscopy showing fewer unpaired spins. Enhanced sensitivity enables detection of single weakly coupled 13C nuclear spins and external 11B spins from a hexagonal boron nitride (h-BN) layer, achieving nanoscale nuclear magnetic resonance. A protective h-BN top layer stabilizes the platform, ensuring robustness against harsh treatments and compatibility with target materials. This integrated approach advances practical quantum sensing by combining extended coherence, improved sensitivity, and device durability.
format Preprint
id arxiv_https___arxiv_org_abs_2507_02312
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Enhancement of quantum coherence in solid-state qubits via interface engineering
Lo, Wing Ki
Zhang, Yaowen
Chow, Ho Yin
Wu, Jiahao
Leung, Man Yin
Ho, Kin On
Du, Xuliang
Chen, Yifan
Shen, Yang
Pan, Ding
Yang, Sen
Mesoscale and Nanoscale Physics
Quantum Physics
Shallow nitrogen-vacancy (NV) centers in diamond are promising quantum sensors but suffer from noise-induced short coherence times due to bulk and surface impurities. We present interfacial engineering via oxygen termination and graphene patching, extending shallow NV coherence to over 1 ms, approaching the T1 limit. Raman spectroscopy and density-functional theory reveal surface termination-driven graphene charge transfer reduces spin noise by pairing surface electrons, supported by double electron-electron resonance spectroscopy showing fewer unpaired spins. Enhanced sensitivity enables detection of single weakly coupled 13C nuclear spins and external 11B spins from a hexagonal boron nitride (h-BN) layer, achieving nanoscale nuclear magnetic resonance. A protective h-BN top layer stabilizes the platform, ensuring robustness against harsh treatments and compatibility with target materials. This integrated approach advances practical quantum sensing by combining extended coherence, improved sensitivity, and device durability.
title Enhancement of quantum coherence in solid-state qubits via interface engineering
topic Mesoscale and Nanoscale Physics
Quantum Physics
url https://arxiv.org/abs/2507.02312