Interplay of frustration and quantum fluctuations in a spin-1/2 anisotropic square lattice

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Autori principali: Ramos, L. M., Zimmer, F. M., Schmidt, M.
Natura: Preprint
Pubblicazione: 2025
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author Ramos, L. M.
Zimmer, F. M.
Schmidt, M.
author_facet Ramos, L. M.
Zimmer, F. M.
Schmidt, M.
contents Motivated by theoretical and experimental studies reported by Yamaguchi et al. (Phys. Rev. B 98, 094402 (2018)), we performed a cluster mean-field analysis of an anisotropic Heisenberg model with six competing exchange interactions. We study the ground and thermal states by tuning the spin anisotropy, magnetic field, and temperature. Our results show that an external magnetic field induces quantum fluctuations, suppressing local moments and leading to the occurrence of a magnetization plateaulike state. When weak spin anisotropy is considered, the competing interactions are affected, and the field-induced fluctuations can lead to a well-defined magnetization plateau within a field range, in which an exotic quantum state can emerge. This state exhibits the coexistence of ferromagnetic and dimerized chains driven by the relation between frustration and the external field. Moreover, we identify a phase transition from a collinear antiferromagnetic order to a disordered state at a finite temperature. Our findings reveal unconventional magnetic properties at low temperatures that can guide future experimental studies of verdazyl-based compounds with anisotropic exchange interactions.
format Preprint
id arxiv_https___arxiv_org_abs_2507_02623
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Interplay of frustration and quantum fluctuations in a spin-1/2 anisotropic square lattice
Ramos, L. M.
Zimmer, F. M.
Schmidt, M.
Strongly Correlated Electrons
Materials Science
Statistical Mechanics
Motivated by theoretical and experimental studies reported by Yamaguchi et al. (Phys. Rev. B 98, 094402 (2018)), we performed a cluster mean-field analysis of an anisotropic Heisenberg model with six competing exchange interactions. We study the ground and thermal states by tuning the spin anisotropy, magnetic field, and temperature. Our results show that an external magnetic field induces quantum fluctuations, suppressing local moments and leading to the occurrence of a magnetization plateaulike state. When weak spin anisotropy is considered, the competing interactions are affected, and the field-induced fluctuations can lead to a well-defined magnetization plateau within a field range, in which an exotic quantum state can emerge. This state exhibits the coexistence of ferromagnetic and dimerized chains driven by the relation between frustration and the external field. Moreover, we identify a phase transition from a collinear antiferromagnetic order to a disordered state at a finite temperature. Our findings reveal unconventional magnetic properties at low temperatures that can guide future experimental studies of verdazyl-based compounds with anisotropic exchange interactions.
title Interplay of frustration and quantum fluctuations in a spin-1/2 anisotropic square lattice
topic Strongly Correlated Electrons
Materials Science
Statistical Mechanics
url https://arxiv.org/abs/2507.02623