Nonlinear Seebeck effect in Ni$_{81}$Fe$_{19}$|Pt at room temperature

Fuente: arXiv
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Autores principales: Hirata, Y., Kikkawa, T., Arisawa, H., Saitoh, E.
Formato: Preprint
Publicado: 2025
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author Hirata, Y.
Kikkawa, T.
Arisawa, H.
Saitoh, E.
author_facet Hirata, Y.
Kikkawa, T.
Arisawa, H.
Saitoh, E.
contents The nonlinear Seebeck effect, nonlinear conversion of a temperature gradient into an electric current, was observed at room temperature. Based on a second-harmonic lock-in method combined with an a.c. temperature gradient, $\nabla T$, we measured a nonlinear Seebeck voltage in NiFe|Pt bilayers at 300 K, the amplitude of which increases in proportion to $(\nabla T)^2$. We also observed that the nonlinear Seebeck voltage increases as the sample length along the $\nabla T$ direction decreases, showing a characteristic scaling law distinct from the conventional linear Seebeck effect. We developed a phenomenological model for the nonlinear Seebeck effect incorporating the spin-current induced modulation of the Seebeck coefficient, which well reproduces the experimental results.
format Preprint
id arxiv_https___arxiv_org_abs_2507_03249
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Nonlinear Seebeck effect in Ni$_{81}$Fe$_{19}$|Pt at room temperature
Hirata, Y.
Kikkawa, T.
Arisawa, H.
Saitoh, E.
Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
The nonlinear Seebeck effect, nonlinear conversion of a temperature gradient into an electric current, was observed at room temperature. Based on a second-harmonic lock-in method combined with an a.c. temperature gradient, $\nabla T$, we measured a nonlinear Seebeck voltage in NiFe|Pt bilayers at 300 K, the amplitude of which increases in proportion to $(\nabla T)^2$. We also observed that the nonlinear Seebeck voltage increases as the sample length along the $\nabla T$ direction decreases, showing a characteristic scaling law distinct from the conventional linear Seebeck effect. We developed a phenomenological model for the nonlinear Seebeck effect incorporating the spin-current induced modulation of the Seebeck coefficient, which well reproduces the experimental results.
title Nonlinear Seebeck effect in Ni$_{81}$Fe$_{19}$|Pt at room temperature
topic Strongly Correlated Electrons
Mesoscale and Nanoscale Physics
Materials Science
url https://arxiv.org/abs/2507.03249