Mode-dependent Emission Thresholds and Frequencies in Metal Nanoparticles within Gain-enhanced Media

Fuente: arXiv
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Hauptverfasser: Caicedo, Karen, Recalde, Nicole, Mora, Milena, Moreta, Alonso, Iatì, Maria Antonia, Maragò, Onofrio M., Infusino, Melissa, Veltri, Alessandro
Format: Preprint
Veröffentlicht: 2025
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author Caicedo, Karen
Recalde, Nicole
Mora, Milena
Moreta, Alonso
Iatì, Maria Antonia
Maragò, Onofrio M.
Infusino, Melissa
Veltri, Alessandro
author_facet Caicedo, Karen
Recalde, Nicole
Mora, Milena
Moreta, Alonso
Iatì, Maria Antonia
Maragò, Onofrio M.
Infusino, Melissa
Veltri, Alessandro
contents We present a mode-resolved analysis of emission thresholds in metal nanoparticles embedded within an infinite gain medium, using Mie scattering theory as a rigorous framework. Focusing on the first three resonant modes, we identify the onset of emission by locating the complex zeros of the electric scattering coefficient a_n(omega), which serve as indicators of lasing conditions. Our hybrid numerical scheme-combining coarse bracketing and two-dimensional Newton refinement-enables precise determination of both the threshold gain G_th,n and the corresponding emission frequency omega_th,n across varying particle radii. The results uncover strong size-dependent behavior, with higher-order modes in larger particles exhibiting significantly reduced threshold gain. These insights elucidate the modal dynamics underlying plasmonic nanolasing and provide design guidelines for active photonic systems leveraging gain-enhanced nanoparticles.
format Preprint
id arxiv_https___arxiv_org_abs_2507_03601
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Mode-dependent Emission Thresholds and Frequencies in Metal Nanoparticles within Gain-enhanced Media
Caicedo, Karen
Recalde, Nicole
Mora, Milena
Moreta, Alonso
Iatì, Maria Antonia
Maragò, Onofrio M.
Infusino, Melissa
Veltri, Alessandro
Optics
We present a mode-resolved analysis of emission thresholds in metal nanoparticles embedded within an infinite gain medium, using Mie scattering theory as a rigorous framework. Focusing on the first three resonant modes, we identify the onset of emission by locating the complex zeros of the electric scattering coefficient a_n(omega), which serve as indicators of lasing conditions. Our hybrid numerical scheme-combining coarse bracketing and two-dimensional Newton refinement-enables precise determination of both the threshold gain G_th,n and the corresponding emission frequency omega_th,n across varying particle radii. The results uncover strong size-dependent behavior, with higher-order modes in larger particles exhibiting significantly reduced threshold gain. These insights elucidate the modal dynamics underlying plasmonic nanolasing and provide design guidelines for active photonic systems leveraging gain-enhanced nanoparticles.
title Mode-dependent Emission Thresholds and Frequencies in Metal Nanoparticles within Gain-enhanced Media
topic Optics
url https://arxiv.org/abs/2507.03601