Nonvolatile Nematic Order Manipulated by Strain and Magnetic Field in a Layered Antiferromagnet

Fuente: arXiv
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Autori principali: Feng, Zili, Lu, Weihang, Lu, Tao, Liu, Fangyan, Sheeran, Joseph R., Ye, Mengxing, Xia, Jing, Kurumaji, Takashi, Ye, Linda
Natura: Preprint
Pubblicazione: 2025
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author Feng, Zili
Lu, Weihang
Lu, Tao
Liu, Fangyan
Sheeran, Joseph R.
Ye, Mengxing
Xia, Jing
Kurumaji, Takashi
Ye, Linda
author_facet Feng, Zili
Lu, Weihang
Lu, Tao
Liu, Fangyan
Sheeran, Joseph R.
Ye, Mengxing
Xia, Jing
Kurumaji, Takashi
Ye, Linda
contents The operation mechanism of nematic liquid crystals lies in the control of their optical properties by the orientation of underlying nematic directors. In analogy, electronic nematicity refers to a state whose electronic properties spontaneously break rotation symmetries of the host crystalline lattice, leading to anisotropic electronic properties. In this work, we demonstrate that the layered antiferromagnet CoTa$_3$S$_6$ exhibits a switchable nematic order, evidenced by the emergence of both resistivity anisotropy and optical birefringence. This nematic state sets in at a temperature $T^*$ distinct from that of the antiferromagnetic transitions in the system, indicating a separate symmetry-breaking mechanism. The nematic order can be manipulated either by an in-plane rotation symmetry-breaking strain or in-plane magnetic field, with the latter exhibiting a pronounced non-volatile memory effect. Remarkably, we find that the broken three-fold rotation symmetry in electronic transport is restored with a moderate out-of-plane field. We hypothesize that the nematicity is of electronic origin and emerges from instabilities associated with van Hove singularities. The resulting phase diagram points to an intertwined interplay between the electronic nematicity and the proposed underlying collinear and non-coplanar spin orders. Our findings establish CoTa$_3$S$_6$ as a versatile antiferromagnetic platform with highly tunable functionalities arising from the breaking of rotational, time-reversal, and inversion symmetries.
format Preprint
id arxiv_https___arxiv_org_abs_2507_05486
institution arXiv
publishDate 2025
record_format arxiv
spellingShingle Nonvolatile Nematic Order Manipulated by Strain and Magnetic Field in a Layered Antiferromagnet
Feng, Zili
Lu, Weihang
Lu, Tao
Liu, Fangyan
Sheeran, Joseph R.
Ye, Mengxing
Xia, Jing
Kurumaji, Takashi
Ye, Linda
Strongly Correlated Electrons
The operation mechanism of nematic liquid crystals lies in the control of their optical properties by the orientation of underlying nematic directors. In analogy, electronic nematicity refers to a state whose electronic properties spontaneously break rotation symmetries of the host crystalline lattice, leading to anisotropic electronic properties. In this work, we demonstrate that the layered antiferromagnet CoTa$_3$S$_6$ exhibits a switchable nematic order, evidenced by the emergence of both resistivity anisotropy and optical birefringence. This nematic state sets in at a temperature $T^*$ distinct from that of the antiferromagnetic transitions in the system, indicating a separate symmetry-breaking mechanism. The nematic order can be manipulated either by an in-plane rotation symmetry-breaking strain or in-plane magnetic field, with the latter exhibiting a pronounced non-volatile memory effect. Remarkably, we find that the broken three-fold rotation symmetry in electronic transport is restored with a moderate out-of-plane field. We hypothesize that the nematicity is of electronic origin and emerges from instabilities associated with van Hove singularities. The resulting phase diagram points to an intertwined interplay between the electronic nematicity and the proposed underlying collinear and non-coplanar spin orders. Our findings establish CoTa$_3$S$_6$ as a versatile antiferromagnetic platform with highly tunable functionalities arising from the breaking of rotational, time-reversal, and inversion symmetries.
title Nonvolatile Nematic Order Manipulated by Strain and Magnetic Field in a Layered Antiferromagnet
topic Strongly Correlated Electrons
url https://arxiv.org/abs/2507.05486